期刊
CHINESE CHEMICAL LETTERS
卷 32, 期 12, 页码 3771-3781出版社
ELSEVIER SCIENCE INC
DOI: 10.1016/j.cclet.2021.05.032
关键词
Single-atom site catalysts; Two-dimensional materials; Synthesis; Characterization; Energy applications
资金
- Science and Technology Key Project of Guangdong Province of China [2020B010188002]
- National Key R&D Program of China [2018YFA0702003]
- National Natural Science Foundation of China [21890383, 21871159]
This review discusses the combination of single-atom site catalysts (SACs) and two-dimensional materials (2DM) in catalysis, highlighting their applications in energy conversion, synthesis, and characterization methods for SACs supported on 2DM, and summarizing the current challenges and perspectives.
Single-atom site catalysts (SACs) and two-dimensional materials (2DM) have gradually become two hot topics in catalysis over the past decades. Their combination with each other can further endow the derived SACs with extraordinary properties such as high loading, identical active sites, uniform coordination environment, distinctive metal-support interaction, and enhanced catalytic activities. In this review, we highlight the recent development in this specific research topic according to the types of substrates and focus on their applications in energy conversion field. Additionally, we also make a brief introduction to the synthesis and characterization methods for SACs supported on 2DM (SACs/2DM). Finally, the challenges and perspectives are summarized based on the current development status. It is believed that this work will make contributions to the rational design and fabrication of novel SACs/2DM, promoting their practical energy applications in the future. (C) 2021 Published by Elsevier B.V. on behalf of Chinese Chemical Society and Institute of Materia Medica, Chinese Academy of Medical Sciences.
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