4.7 Article

CoFe-LDH nanowire arrays on graphite felt: A high-performance oxygen evolution electrocatalyst in alkaline media

期刊

CHINESE CHEMICAL LETTERS
卷 33, 期 2, 页码 890-892

出版社

ELSEVIER SCIENCE INC
DOI: 10.1016/j.cclet.2021.10.002

关键词

LDH; Graphite felt; Electrocatalyst; Oxygen evolution; Alkaline media

资金

  1. National Natural Science Foundation of China [22072015]

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This research fabricates CoFe-layered double hydroxide (LDH) nanowire arrays on graphite felt (CoFe-LDH/GF) through a hydrothermal method, producing a high-performance non-noble-metal oxygen evolution reaction (OER) electrocatalyst with excellent catalytic activity, low overpotential, and electrochemical durability, providing new possibilities for the development of attractive catalyst supports for oxygen evolution applications.
Developing non-noble-metal oxygen evolution reaction (OER) electrocatalysts with high performance is critical to electrocatalytic water splitting. In this work, we fabricated CoFe-layered double hydroxide (LDH) nanowire arrays on graphite felt (CoFe-LDH/GF) via a hydrothermal method. The CoFe-LDH/GF, as a robust integrated 3D OER anode, exhibits excellent catalytic activity with the need of low overpotential of 252 and 285 mV to drive current densities of 10 and 100 mA/cm(2) in 1.0 mol/L KOH, respectively. In addition, it also maintains electrochemical durability for at least 24 h. This work would open up avenues for the development of GF like attractive catalyst supports for oxygen evolution applications. (C) 2021 Published by Elsevier B.V. on behalf of Chinese Chemical Society and Institute of Materia Medica, Chinese Academy of Medical Sciences.

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