☆ 4.8 Review

MOF-enabled confinement and related effects for chemical catalyst presentation and utilization

CHEMICAL SOCIETY REVIEWS (2022)

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A Metal-Organic Framework (MOF)-Based Multifunctional Cargo Vehicle for Reactive-Gas Delivery and Catalysis

Preecha Kittikhunnatham et al.

Summary: This study investigated the efficient delivery of reactive and toxic gaseous reagents in organic reactions using metal-organic frameworks (MOFs). It was found that MOFs can serve as both gas cargo vehicles and catalysts, leading to high product yields. Moreover, the MOFs can be recycled without sacrificing product yield and crystallinity, indicating the potential of developing multifunctional MOF-based reagent-catalyst cargo vessels as an attractive alternative to toxic pure gases or gas generators.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Chemistry, Physical

Mechanism-Guided Design of Metal-Organic Framework Composites for Selective Photooxidation of a Mustard Gas Simulant under Solvent-Free Conditions

Yajiao Hao et al.

Summary: Photoactive metal-organic frameworks and their derivatives show promise in selectively oxidizing toxic organic sulfides under visible or UV light. By stabilizing a persulfoxide intermediate with hydrogen-bond donors, a series of MOF/textile composites were developed for selective photooxidation of organic sulfides under solvent-free conditions. These composites achieved rapid, selective, and solvent-free degradation of mustard gas simulants with excellent stability and reusability.

ACS CATALYSIS (2022)

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Article Chemistry, Applied

Co-catalyst free ethene dimerization over Zr-based metal-organic framework (UiO-67) functionalized with Ni and bipyridine

Mustafa Komurcu et al.

Summary: Nickel-functionalized metal organic frameworks (MOFs) show promising catalytic performance in ethene dimerization, but often require a large amount of co-catalyst. A novel Ni(II)-bpy functionalized UiO-67 MOF was reported in this study for efficient ethene dimerization reaction without the need for a co-catalyst, yielding highly selective linear butenes.

CATALYSIS TODAY (2021)

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Article Chemistry, Multidisciplinary

Zr-MOF-808 as Catalyst for Amide Esterification

Beatriz Villoria-del-Alamo et al.

Summary: Zr-MOF-808-P has been identified as an efficient and versatile catalyst for amide esterification, demonstrating the ability to promote a wide range of reactions with different primary, secondary, and tertiary amides. The catalyst acts as a heterogeneous catalyst, allowing for at least five consecutive cycles of reuse, and has been studied at a molecular level for the amide esterification mechanism.

CHEMISTRY-A EUROPEAN JOURNAL (2021)

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Review Chemistry, Inorganic & Nuclear

A historical perspective on porphyrin-based metal-organic frameworks and their applications

Xuan Zhang et al.

Summary: Porphyrins are important molecules widely found in nature, and recent interest in using them as building blocks for metal-organic frameworks has increased rapidly. Porphyrin-based MOFs with atomically precise structures provide an ideal platform for studying structure-function relationships in the solid state without compromising the inherent properties of the porphyrin building blocks.

COORDINATION CHEMISTRY REVIEWS (2021)

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Review Nanoscience & Nanotechnology

Confining isolated atoms and clusters in crystalline porous materials for catalysis

Lichen Liu et al.

Summary: This review discusses the impact of confining subnanometric metal species in zeolites and metal-organic frameworks on their geometric and electronic structures, as well as catalytic performance. It also highlights the potential of the interaction between metal species and porous frameworks in modulating the properties of subnanometric metal species. Future research directions in this area are proposed for further exploration.

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Article Chemistry, Physical

Exploitation of Intrinsic Confinement Effects of MOFs in Catalysis

Karina Hemmer et al.

Summary: The importance of designing bio-inspired "artificial enzymes" in catalysis research is highlighted, with a focus on the use of metal-organic frameworks (MOFs) to achieve this goal. The potential of exploiting the confinement effects of MOFs for the design of sophisticated catalysts is emphasized in controlling catalytic activity and selectivity.

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Review Chemistry, Multidisciplinary

Metal-Organic Framework-Based Enzyme Biocomposites

Weibin Liang et al.

Summary: Enzymes play a crucial role in chemical synthesis and biotechnology, but their activity can be easily affected by external stressors. Metal-organic frameworks (MOFs) offer protection to enzymes through encapsulation or infiltration, allowing them to maintain activity under challenging conditions.

CHEMICAL REVIEWS (2021)

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Review Chemistry, Inorganic & Nuclear

Recent advances in the synthesis techniques for zeolitic imidazolate frameworks and their sensing applications

Preeti Kukkar et al.

Summary: Zeolitic imidazolate frameworks (ZIFs) belong to metal-organic frameworks (MOFs) or metalazolate frameworks (MAFs) with unique topologies, allowing for robust coordination and advantageous properties such as easy crystallization, high loading capacities, and good biocompatibility. Technical advancements in porous coordination polymers synthesis have diversified fabrication approaches for ZIFs, leading to the characterization of their structural and functional attributes.

COORDINATION CHEMISTRY REVIEWS (2021)

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Review Chemistry, Inorganic & Nuclear

Chiral metal-organic frameworks based on asymmetric synthetic strategies and applications

Zahra Sharifzadeh et al.

Summary: Chiral metal-organic frameworks (CMOFs) have attracted considerable attention as chiral porous materials for asymmetric catalysis and ferroelectricity applications. Despite various studies on CMOFs, further research on enantioselective catalysis is limited, presenting opportunities for future exploration.

COORDINATION CHEMISTRY REVIEWS (2021)

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Article Chemistry, Multidisciplinary

Rational Construction of an Artificial Binuclear Copper Monooxygenase in a Metal-Organic Framework

Xuanyu Feng et al.

Summary: A novel strategy for constructing an artificial binuclear copper monooxygenase starting from a Ti metal-organic framework was reported. Experimental and computational studies showed that the enzyme exhibited outstanding catalytic activity in monoxygenation processes and significantly higher activity compared to a mononuclear copper monooxygenase. This was attributed to the cooperative stabilization of Cu-O-2 adduct by Cu-2 sites, leading to a lower free energy increase for O-O bond cleavage.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Multidisciplinary

Peptide-Metal Frameworks with Metal Strings Guided by Dispersion Interactions

Tobias Schnitzer et al.

Summary: Despite the challenges in forming networks from peptidic ligands, a peptide-metal framework consisting of helical oligoproline ligands and Zn/K (or Zn/Rb) has been successfully created in this study. The crystal network contains pleated nanosheets with metal ions aligned in strings, with the unique architecture derived from under-appreciated London dispersion interactions between the ligands. The secondary structure of the peptidic ligand plays an important role in the creation of new MOF architectures.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Editorial Material Chemistry, Inorganic & Nuclear

Pioneers and Influencers in Organometallic Chemistry: Professor Robert Crabtree's Storied Career via an Unusual Journey to the Ivy League

Graham E. Dobereiner et al.

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Article Chemistry, Physical

Rapid, Biomimetic Degradation of a Nerve Agent Simulant by Incorporating Imidazole Bases into a Metal-Organic Framework

Hong-Bin Luo et al.

Summary: A new synthetic strategy has been developed to synthesize MOF composites for efficient degradation of nerve agent simulants without the need for liquid base. One of the composites, Im@MOF-808, exhibited the highest catalytic activity for DMNP hydrolysis in unbuffered aqueous solutions. This research provides a viable solution for the practical implementation of MOF materials in protective equipment for nerve agent detoxification.

ACS CATALYSIS (2021)

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Article Chemistry, Physical

Influence of First and Second Coordination Environment on Structural Fe(II) Sites in MIL-101 for C-H Bond Activation in Methane

Jenny G. Vitillo et al.

Summary: The study demonstrates that modifying the microenvironment around the divalent iron sites in metal-organic frameworks can modulate their catalytic activity for light alkane oxidation. By varying substituents and their proximity to the active site, the stability and reactivity of the Fe(IV)=O species can be improved to lower energy barriers for methane oxidation to methanol reaction.

ACS CATALYSIS (2021)

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Article Chemistry, Physical

Integration of Earth-Abundant Photosensitizers and Catalysts in Metal-Organic Frameworks Enhances Photocatalytic Aerobic Oxidation

Xuanyu Feng et al.

Summary: In this study, two metal-organic frameworks were constructed to facilitate the photocatalytic oxidation reactions of copper and iron. The materials showed high catalytic efficiency and good recyclability. Analysis of the photooxidation mechanism provided insights into the catalytic mechanism.

ACS CATALYSIS (2021)

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Article Chemistry, Multidisciplinary

High Ammonia Adsorption in MFM-300 Materials: Dynamics and Charge Transfer in Host-Guest Binding

Xue Han et al.

Summary: A series of robust metal-organic framework materials show high NH3 adsorption capacity, with V-IV exhibiting the highest uptake. The redox-active V center enables charge transfer between host and guest, leading to the oxidation of NH3 to hydrazine. The combination of in situ techniques and modeling provides insights into the binding dynamics of adsorbed NH3 within these MOFs.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Nanoscience & Nanotechnology

Ammonia Capture within Zirconium Metal-Organic Frameworks: Reversible and Irreversible Uptake

Jian Liu et al.

Summary: The research found that ammonia can be adsorbed by zirconium-based metal-organic framework material NU-1000 through both physisorption and chemisorption, with reversible and irreversible processes. Different adsorption modes are influenced by thermal treatment and structural distortion.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Nanoscience & Nanotechnology

Zirconium Metal-Organic Frameworks Integrating Chloride Ions for Ammonia Capture and/or Chemical Separation

Jian Liu et al.

Summary: The study found that NU-1000-Cl has enhanced capacity for both reversible and irreversible uptake of ammonia compared to the chloride-free version. The presence of chloride ions also facilitates irreversible reactions between ammonia and NU-1000-Cl. The chemical interactions between ammonia and NU1000-Cl result in the separation of NH3 from N-2 at room temperature.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Review Chemistry, Physical

Connecting theory and simulation with experiment for the study of diffusion in nanoporous solids

Brandon C. Bukowski et al.

Summary: Nanoporous solids are essential for chemical, energy, and environmental processes, with a variety of materials such as crystalline microporous zeotypes, metal-organic frameworks, and mesoporous and hierarchically structured materials playing crucial roles. Molecular simulation techniques combined with experimental measurements have been successful in studying diffusion processes within nanoporous solids. Future developments and experimental techniques are needed for more accurate predictions in complex systems.

ADSORPTION-JOURNAL OF THE INTERNATIONAL ADSORPTION SOCIETY (2021)

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Article Chemistry, Physical

PMo12@UiO-67 nanocomposite as a novel non-leaching catalyst with enhanced performance durability for sulfur removal from liquid fuels with exceptionally diluted oxidant

Reza Abazari et al.

Summary: In this study, a novel heterogeneous catalyst was developed for the removal of sulfur compounds, showing high catalytic activity and good recyclability.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Chemistry, Physical

Deciphering the oxygen activation mechanism at the CuC site of particulate methane monooxygenase

Wei Peng et al.

Summary: This study deciphers the catalytic cycle of pMMO in the presence of the physiological reductant duroquinol (DQH(2)), revealing that O-2 activation is initiated by the Cu-C(ii)-DQH(-) species. The research also uncovers the important roles of the phenol co-substrate for O-2 activation.

NATURE CATALYSIS (2021)

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Article Nanoscience & Nanotechnology

Engineering Dendrimer-Templated, Metal-Organic Framework-Confined Zero-Valent, Transition-Metal Catalysts

Ying Yang et al.

Summary: A strategy for synthesizing sub-nanometer to 2 nm metal clusters and particles was successfully demonstrated, utilizing a combination of a metal-organic framework (MOF) and dendrimer templates to improve synthesis and create stable, efficient heterogeneous catalysts.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Metalloenzyme-Inspired Ce-MOF Catalyst for Oxidative Halogenation Reactions

Sergio Rojas-Buzo et al.

Summary: The structure of UiO-66(Ce) consists of CeO2-x defective nanoclusters linked by terephthalate ligands, facilitating charge transfer and resulting in higher oxidase-like activity compared to nanoceria under aerobic conditions. Ce-based metal-organic frameworks (MOFs) show promising potential as efficient catalysts for oxidative halogenation reactions, with UiO-66(Ce) demonstrating at least three times greater activity and excellent stability compared to nanoceria, while also mimicking the mechanistic pathway of metalloenzymes.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Product Inhibition and the Catalytic Destruction of a Nerve Agent Simulant by Zirconium-Based Metal-Organic Frameworks

Yijun Liao et al.

Summary: This study investigates the effects of product inhibition on catalytic activity in the degradation of chemical warfare agents, particularly those containing a phosphorous-fluorine bond. Results indicate substantial product inhibition on catalyst activity after several turnovers, with apparent product binding constants obtained to quantitatively describe the inhibition effects over time. The study highlights the importance of understanding product inhibition in the catalytic hydrolysis of chemical warfare agents.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Review Chemistry, Multidisciplinary

Metal-Organic Framework-Based Hierarchically Porous Materials: Synthesis and Applications

Guorui Cai et al.

Summary: Metal-organic frameworks (MOFs) are fascinating materials with high porosity and tailored structures, but their narrow pores limit applications. The development of hierarchically porous MOFs and derivatives has attracted attention to broaden the scope of traditional MOF-based materials.

CHEMICAL REVIEWS (2021)

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Article Chemistry, Physical

Art of Architecture: Efficient Transport through Solvent-Filled Metal-Organic Frameworks Regulated by Topology

Rui Wang et al.

Summary: This study investigated the transport of guest molecules through two Zr-MOFs with different topologies, NU-600 and NU-1008. It was found that the she-net NU-600 provided more efficient pathways for substrate transport compared to the csq-net NU-1008. The differences in morphology and structure were crucial in determining the transport efficiency advantages of NU-600. Additionally, atomistic simulations showed energetically favorable interactions between the linkers and dye molecules, supporting the experimental findings of lower diffusivity in NU-600.

CHEMISTRY OF MATERIALS (2021)

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Review Chemistry, Inorganic & Nuclear

Computational catalysis for metal-organic frameworks: An overview

Gavin A. McCarver et al.

Summary: Metal-organic frameworks (MOFs) show great promise in the field of catalysis, acting as both active catalysts and supporting materials. Recent research focuses on computational and theoretical aspects of catalytic reactions, including elucidating reaction mechanisms, characterizing electronic structure effects, and interpreting experimental data. Studies aim to understand structure-function relations and design new MOF catalysts, with future prospects involving high-throughput virtual screening and machine learning methods.

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Review Chemistry, Multidisciplinary

Metal-Organic Framework UiO-68 and Its Derivatives with Sufficiently Good Properties and Performance Show Promising Prospects in Potential Industrial Applications

Xin Ye et al.

Summary: UiO-68 is a Zr-based metal-organic framework with high surface area, exceptional thermal stability, and remaining crystalline at high pressure, making it promising for industrial applications. By adjusting the organic linkers, UiO-68 with desired functionalities can be obtained. UiO-68 and its derivatives have various applications such as catalysts, sorbents, drug delivery, fluorescent probes, and sensors.

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Article Chemistry, Multidisciplinary

Transport Diffusion of Linear Alkanes (C5-C16) through Thin Films of ZIF-8 as Assessed by Quartz Crystal Microgravimetry

Cornelius O. Audu et al.

Summary: The study found that the transport dynamics in ZIF-8 are mainly governed by guest diffusion through the metal-organic framework rather than entry into the film. Additionally, the increase in carbon atoms leads to a halving of the transport diffusivity of alkanes, and an odd-even effect was observed where alkanes with even numbers of carbons diffuse more rapidly.

LANGMUIR (2021)

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Article Chemistry, Multidisciplinary

Boosting Catalytic Efficiency of Metal-Organic Frameworks with Electron-Withdrawing Effect for Lewis-Acid Catalysis

Siyu Li et al.

Summary: Metal Organic Frameworks (MOFs) with high specific surface area and abundant active sites are emerging as versatile heterogeneous catalysts. By synthesizing MOFs with different substituents and evaluating their catalytic activity, the study found that MIL-101(Fe)-NO2 exhibited the best conversion rate due to its electron withdrawing effect. This demonstrates the versatility of electronic effects on catalytic activity and the potential for tuning MOFs activity through introduction of different organic ligands.

CHEMISTRYSELECT (2021)

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Review Chemistry, Multidisciplinary

The chemistry and applications of hafnium and cerium(iv) metal-organic frameworks

Zhigang Hu et al.

Summary: Metal-organic frameworks (MOFs) are formed by the coordination connection of organic linkers to metal clusters, with tunable ligands providing robust molecular porosity. Hafnium (Hf) and tetravalent cerium [Ce(iv)] MOFs have shown promise for practical applications, with a focus on their chemistry, topologies, synthetic strategies, and diverse applications. Future research will explore the development of Hf/Ce-MOFs, including fundamental design, defect engineering, and computational approaches for tailor-made applications.

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Immobilization of Rh(I) precursor in a porphyrin metal-organic framework - turning on the catalytic activity

Anna M. Szczepkowska et al.

Summary: Two model porphyrin metal-organic frameworks were utilized for the incorporation of Rh(I) species through post-synthetic metallation, resulting in the synthesis and structural characterization of new rhodium MOFs (Rh/MOFs), Rh/PCN-222 and Rh/NU-1102. These Rh/MOFs were demonstrated to be active heterogeneous catalysts for the hydrogenation of unsaturated hydrocarbons at mild reaction conditions, with an activation step required during the initial run of the catalytic process. In situ Diffuse Reflectance Infrared Fourier Transform Spectroscopy (DRIFTS) was utilized to monitor the activation pathway of the catalyst under a H-2 atmosphere.

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Computational determination of coordination structure impact on adsorption and acidity of pristine and sulfated MOF-808

Bo Yang et al.

Summary: Metal-organic frameworks (MOFs) consist of metal nodes connected by organic linkers with a wide range of possible metal and linker combinations. Computational analysis of coordination structures in MOF-808 and sulfated MOF-808 provides insights into their physical and chemical properties, highlighting the importance of structure-property relationships in MOFs.

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Towards a unified understanding of the copper sites in particulate methane monooxygenase: an X-ray absorption spectroscopic investigation†

George E. Cutsail et al.

Summary: The study investigated the enzymatic conversion of methane to methanol by methane monooxygenases (MMOs) under mild conditions. The results revealed the presence of only monocopper sites in particulate MMO (pMMO), contradicting the previous proposed dicopper site. Additionally, photodamage was found to partially contribute to observed features in X-ray absorption spectrum, highlighting the complexity involved in EXAFS measurement and modeling of dilute metalloproteins with multiple metal centers.

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Review Chemistry, Multidisciplinary

Heterogenisation of polyoxometalates and other metal-based complexes in metal-organic frameworks: from synthesis to characterisation and applications in catalysis

P. Mialane et al.

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A cofacial metal-organic framework based photocathode for carbon dioxide reduction

Bowen Ding et al.

Summary: Innovative and robust photosensitisation materials in the form of Metal-Organic Frameworks (MOFs) have been shown to lower the overpotential required for CO2 reduction to CO, along with facilitating charge transfer reduction of a rhenium molecular electrocatalyst, ultimately leading to lower overpotential for CO generation. This study demonstrates the importance of through-space Intervalence Charge Transfer (IVCT) within cofacial units in MOFs in achieving light-harvesting functionalities, offering new directions for the design philosophy behind such materials.

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Shaoyang Lin et al.

Summary: The mixed-linker MOF film combines photosensitizer and catalyst, increasing catalytic efficiency due to the activation of the photosensitizer. Furthermore, energy and/or electron transfer during the photochemical process also play a role in enhancing catalytic efficiency.

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A Decade of UiO-66 Research: A Historic Review of Dynamic Structure, Synthesis Mechanisms, and Characterization Techniques of an Archetypal Metal-Organic Framework

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In Situ Imine-Based Linker Formation for the Synthesis of Zirconium MOFs: A Route to CO2 Capture Materials and Ethylene Oligomerization Catalysts

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On the Electronic and Optical Properties of Metal-Organic Frameworks: Case Study of MIL-125 and MIL-125-NH2

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Hydrogenation of CO2 to Methanol by Pt Nanoparticles Encapsulated in UiO-67: Deciphering the Role of the Metal-Organic Framework

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Engineering a Highly Defective Stable UiO-66 with Tunable Lewis-Bronsted Acidity: The Role of the Hemilabile Linker

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Integration of Enzymes and Photosensitizers in a Hierarchical Mesoporous Metal-Organic Framework for Light-Driven CO2 Reduction

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Photoactivation of Cu Centers in Metal-Organic Frameworks for Selective CO2 Conversion to Ethanol

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A Smart Route for Encapsulating Pd Nanoparticles into a ZIF-8 Hollow Microsphere and Their Superior Catalytic Properties

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Ligand-Functionalization-Controlled Activity of Metal-Organic Framework-Encapsulated Pt Nanocatalyst toward Activation of Water

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Synthesis of Chiral MOF-74 Frameworks by Post-Synthetic Modification by Using an Amino Acid

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Quantum Chemical Characterization of Structural Single Fe(II) Sites in MIL-Type Metal-Organic Frameworks for the Oxidation of Methane to Methanol and Ethane to Ethanol

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Accelerated Computational Analysis of Metal-Organic Frameworks for Oxidation Catalysis

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Metal-Organic Frameworks Stabilize Mono(phosphine)-Metal Complexes for Broad-Scope Catalytic Reactions

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Metal-Organic Frameworks Stabilize Solution-Inaccessible Cobalt Catalysts for Highly Efficient Broad-Scope Organic Transformations

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Rhodium Hydrogenation Catalysts Supported in Metal Organic Frameworks: Influence of the Framework on Catalytic Activity and Selectivity

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Dynamic Release-Immobilization of a Homogeneous Rhodium Hydroformylation Catalyst by a Polyoxometalate Metal-Organic Framework Composite

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Co@NH2-MIL-125(Ti): cobaloxime-derived metal-organic framework-based composite for light-driven H-2 production

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Spatial Confinement of a Co3O4 Catalyst in Hollow Metal-Organic Frameworks as a Nanoreactor for Improved Degradation of Organic Pollutants

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Photocatalytic CO2 Reduction to Formate Using a Mn(I) Molecular Catalyst in a Robust Metal-Organic Framework

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Immobilization of Cu Complex into Zr-Based MOF with Bipyridine Units for Heterogeneous Selective Oxidation

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Bias-Switchable Permselectivity and Redox Catalytic Activity of a Ferrocene-Functionalized, Thin-Film Metal-Organic Framework Compound

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Bupyridine- and Phenanthroline-Based Metal-Organic Frameworks for Highly Efficient and Tandem Catalytic Organic Transformations via Directed C-H Activation

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Fe-Porphyrin-Based Metal-Organic Framework Films as High-Surface Concentration, Heterogeneous Catalysts for Electrochemical Reduction of CO2

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Gas-Phase Dimerization of Ethylene under Mild Conditions Catalyzed by MOF Materials Containing (bpy)NiII Complexes

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Pt@ZIF-8 composite for the regioselective hydrogenation of terminal unsaturations in 1,3-dienes and alkynes

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Cr-MIL-101 encapsulated Keggin phosphotungstic acid as active nanomaterial for catalysing the alcoholysis of styrene oxide

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Why Does Enzyme Not Leach from Metal-Organic Frameworks (MOFs)? Unveiling the Interactions between an Enzyme Molecule and a MOF

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Manganese Catalysts with Bulky Bipyridine Ligands for the Electrocatalytic Reduction of Carbon Dioxide: Eliminating Dimerization and Altering Catalysis

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Postsynthetic Metalation of Bipyridyl-Containing Metal-Organic Frameworks for Highly Efficient Catalytic Organic Transformations

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Molecular Encapsulation beyond the Aperture Size Limit through Dissociative Linker Exchange in Metal-Organic Framework Crystals

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One-Pot Synthesis of Protein-Embedded Metal-Organic Frameworks with Enhanced Biological Activities

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Semisynthetic Artemisinin, the Chemical Path to Industrial Production

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Pt Nanoclusters Confined within Metal Organic Framework Cavities for Chemoselective Cinnamaldehyde Hydrogenation

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ACS CATALYSIS (2014)

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Heterogeneous Catalysis for Tandem Reactions

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Zeolitic imidazolate framework materials: recent progress in synthesis and applications

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Adsorption/catalytic properties of MIL-125 and NH2-MIL-125

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CATALYSIS TODAY (2013)

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A robust amino-functionalized titanium(IV) based MOF for improved separation of acid gases

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Alcohol and water adsorption in zeolitic imidazolate frameworks

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Oxygen Defects and Surface Chemistry of Ceria: Quantum Chemical Studies Compared to Experiment

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Design, Synthesis, Characterization, and Catalytic Properties of a Large-Pore Metal-Organic Framework Possessing Single-Site Vanadyl(monocatecholate) Moieties

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CRYSTAL GROWTH & DESIGN (2013)

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Structure stability of metal-organic framework MIL-53 (Al) in aqueous solutions

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INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2013)

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Construction of Ultrastable Porphyrin Zr Metal-Organic Frameworks through Linker Elimination

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Systematic Modulation of Quantum (Electron) Tunneling Behavior by Atomic Layer Deposition on Nanoparticulate SnO2 and TiO2 Photoanodes

Chaiya Prasittichai et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2013)

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Stepwise Transformation of the Molecular Building Blocks in a Porphyrin-Encapsulating Metal-Organic Material

Zhenjie Zhang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2013)

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Heterogenization of Homogeneous Catalysts in Metal-Organic Frameworks via Cation Exchange

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2013)

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Engineering the Optical Response of the Titanium-MIL-125 Metal-Organic Framework through Ligand Functionalization

Christopher H. Hendon et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2013)

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Vapor-Phase Metalation by Atomic Layer Deposition in a Metal-Organic Framework

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2013)

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Review Biochemistry & Molecular Biology

Chemical Reactions Catalyzed by Metalloporphyrin-Based Metal-Organic Frameworks

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A chiral porous metallosalan-organic framework containing titanium-oxo clusters for enantioselective catalytic sulfoxidation

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CHEMICAL SCIENCE (2013)

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Transmetalation: routes to metal exchange within metal-organic frameworks

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Zirconium-Metalloporphyrin PCN-222: Mesoporous Metal-Organic Frameworks with Ultrahigh Stability as Biomimetic Catalysts

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A highly porous metal-organic framework, constructed from a cuboctahedral super-molecular building block, with exceptionally high methane uptake

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CHEMICAL COMMUNICATIONS (2012)

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Evolved Stereoselective Hydrolases for Broad-Spectrum G-Type Nerve Agent Detoxification

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Chromium(III) Terephthalate Metal Organic Framework (MIL-101): HF-Free Synthesis, Structure, Polyoxometalate Composites, and Catalytic Properties

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Titration of Zr3(μ-OH) Hydroxy Groups at the Cornerstones of Bulk MOF UiO-67, [Zr6O4(OH)4(biphenyldicarboxylate)6], and Their Reaction with [AuMe(PMe3)]

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Biomimetic Catalysis of a Porous Iron-Based Metal-Metalloporphyrin Framework

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Synthesis, Structure, and Metalation of Two New Highly Porous Zirconium Metal-Organic Frameworks

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Reversible Alteration of CO2 Adsorption upon Photochemical or Thermal Treatment in a Metal-Organic Framework

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Postsynthetic Ligand and Cation Exchange in Robust Metal-Organic Frameworks

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Pervaporation studies of n-hexane, benzene, mesitylene and their mixtures on zeolitic imidazolate framework-8 membranes

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Imparting functionality to a metal-organic framework material by controlled nanoparticle encapsulation

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NATURE CHEMISTRY (2012)

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Synergistic catalysis: A powerful synthetic strategy for new reaction development

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Metal-adeninate vertices for the construction of an exceptionally porous metal-organic framework

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NATURE COMMUNICATIONS (2012)

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Immobilization of MP-11 into a Mesoporous Metal-Organic Framework, MP-11@mesoMOF: A New Platform for Enzymatic Catalysis

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Doping Metal-Organic Frameworks for Water Oxidation, Carbon Dioxide Reduction, and Organic Photocatalysis

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2011)

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An Exceptional 54-Fold Interpenetrated Coordination Polymer with 103-srs Network Topology

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Synergistic Catalysis of Metal-Organic Framework-Immobilized Au-Pd Nanoparticles in Dehydrogenation of Formic Acid for Chemical Hydrogen Storage

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Opening the Gate: Framework Flexibility in ZIF-8 Explored by Experiments and Simulations

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The Nature of Surface Barriers on Nanoporous Solids Explored by Microimaging of Transient Guest Distributions

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Synthesis, Structure, and Carbon Dioxide Capture Properties of Zeolitic Imidazolate Frameworks

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Engineering Metal Organic Frameworks for Heterogeneous Catalysis

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Metal-Organic Frameworks as Sensors: A ZIF-8 Based Fabry-Perot Device as a Selective Sensor for Chemical Vapors and Gases

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Synthesis of the 2Fe subcluster of the [FeFe]-hydrogenase H cluster on the HydF scaffold

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PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2010)

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Postsynthetic Modification Switches an Achiral Framework to Catalytically Active Homochiral Metal-Organic Porous Materials

Mainak Banerjee et al.

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A New Photoactive Crystalline Highly Porous Titanium(IV) Dicarboxylate

Meenakshi Dan-Hardi et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2009)

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Review Chemistry, Multidisciplinary

Mesoporous materials for encapsulating enzymes

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NANO TODAY (2009)

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Review Chemistry, Multidisciplinary

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NATURE CHEMISTRY (2009)

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The Reticular Chemistry Structure Resource (RCSR) Database of, and Symbols for, Crystal Nets

Michael O'Keeffe et al.

ACCOUNTS OF CHEMICAL RESEARCH (2008)

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Template-Directed Assembly of Zeolite-like Metal-Organic Frameworks (ZMOFs): A usf-ZMOF with an Unprecedented Zeolite Topology

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2008)

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Review Chemistry, Multidisciplinary

Heterogeneous Multifunctional Catalysts for Tandem Processes: An Approach toward Sustainability

Francois-Xavier Felpin et al.

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A new zirconium inorganic building brick forming metal organic frameworks with exceptional stability

Jasmina Hafizovic Cavka et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2008)

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Topotactic linear radical polymerization of divinylbenzenes in porous coordination polymers

Takashi Uemura et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2007)

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Exceptional chemical and thermal stability of zeolitic imidazolate frameworks

Kyo Sung Park et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2006)

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A metal-organic framework material that functions as an enantioselective catalyst for olefin epoxidation

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Nanochannel-promoted polymerization of substituted acetylenes in porous coordination polymers

Takashi Uemura et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2006)

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Homochiral porous metal-organic framework for highly enantioselective heterogeneous asymmetric catalysis

CD Wu et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2005)

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Review Chemistry, Multidisciplinary

Microporous porphyrin solids

KS Suslick et al.

ACCOUNTS OF CHEMICAL RESEARCH (2005)

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Concurrent tandem catalysis

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CHEMICAL REVIEWS (2005)

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Homogeneous and heterogeneous catalysis: Bridging the gap through surface organometallic chemistry

C Coperet et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2003)

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Article Chemistry, Multidisciplinary

Very large breathing effect in the first nanoporous chromium(III)-based solids:: MIL-53 or CrIII(OH)•{O2C-C6H4-CO2}•{HO2C-C6H4-CO2H}x•H2Oy

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Asymmetric allylic oxidation with biarylbisoxazoline-copper(I) catalysis

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