☆ 4.8 Review

Liquid metals: an ideal platform for the synthesis of two-dimensional materials

CHEMICAL SOCIETY REVIEWS (2022)

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Review Chemistry, Multidisciplinary

Stacking of 2D Materials

Hao-Wei Guo et al.

Summary: The stacking technique of 2D layered materials is a powerful strategy to achieve high-quality and controlled structures, with a variety of properties and applications, by artificially assembling different dimensional materials. Factors in the stacking process play a crucial role in determining the structure and properties, such as surface quality, angle control, and sample size.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Self-Deposition of 2D Molybdenum Sulfides on Liquid Metals

Yifang Wang et al.

Summary: The self-deposition of 2D molybdenum sulfide on the surface of EGaIn allows for the formation of large-scale planar molybdenum sulfides, resulting in highly crystalline 2H-MoS(2) after annealing. This work demonstrates a fundamentally new capability for the formation of large-scale 2D TMDs.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Nanoscience & Nanotechnology

Atomically Thin Tin Monoxide-Based p-Channel Thin-Film Transistor and a Low-Power Complementary Inverter

Chi-Hsin Huang et al.

Summary: Research has developed a high-performance p-channel oxide thin-film transistor (TFT) using an atomically thin p-type tin monoxide (SnO) channel, demonstrating good device performance. N-channel oxide TFTs and low-power complementary inverter circuits have been successfully fabricated using metal-liquid printing technology.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Nanoscience & Nanotechnology

Artificial Synapse Based on a 2D-SnO2 Memtransistor with Dynamically Tunable Analog Switching for Neuromorphic Computing

Chi-Hsin Huang et al.

Summary: The study demonstrates a new type of gate-tunable memristor based on 2D-SnO2 material, which can achieve complex neuromorphic learning. By regulating the gate bias, the gate-tunable synaptic device dynamically modulates the analog switching behavior, while exhibiting excellent linearity and an improved conductance change ratio. This new device opens up new opportunities for advancing neuromorphic device technology.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Nanoscience & Nanotechnology

Liquid-Metal-Assisted Deposition and Patterning of Molybdenum Dioxide at Low Temperature

Yifang Wang et al.

Summary: The method presented in the study utilizes liquid metal-based technology to achieve room temperature deposition and patterning of MoO2, providing a new way of fabrication. Through laser writing technique, electrically conductive MoO2 patterns can be obtained on desired substrates. The electrical conductivity and plasmonic properties of MoO2 are analyzed and demonstrated.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

High-k 2D Sb2O3 Made Using a Substrate-Independent and Low-Temperature Liquid-Metal-Based Process

Kibret A. Messalea et al.

Summary: A stoichiometric cubic polymorph of 2D antimony oxide (Sb2O3) was synthesized as an ideal high-k dielectric sheet using a low-temperature, substrate-independent, silicon-industry-compatible liquid metal synthesis technique. The obtained alpha-Sb2O3 exhibited high crystallinity, wide band gap of approximately 4.4 eV, and a maximum relative permittivity of 84 with a breakdown electric field of around 10 MV/cm. The isolated 2D alpha-Sb2O3 nanosheets showed promise as gate oxides for conventional and van der Waals heterostructure-based electronics due to low leakage currents in top-gated field-effect transistors.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

Printable Single-Unit-Cell-Thick Transparent Zinc-Doped Indium Oxides with Efficient Electron Transport Properties

Azmira Jannat et al.

Summary: This research explores the use of transition metal doping in ultrathin In2O3, achieving thickness down to the single-unit-cell limit using low-temperature liquid metal printing. By optimizing Zn doping levels, the material retains high optical transparency, while achieving significantly improved electron field-effect mobility and electrical conductivity.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

Ultrathin Ga2O3 Glass: A Large-Scale Passivation and Protection Material for Monolayer WS2

Matthias Wurdack et al.

Summary: Atomically thin transition metal dichalcogenide crystals have exceptional optical properties. Encapsulation of these crystals in ultrathin Ga2O3 glass can enhance their optical performance and protect them from further material deposition. Ga2O3 is highly suitable for large-scale passivation and protection of monolayer TMDCs in functional heterostructures.

ADVANCED MATERIALS (2021)

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Review Chemistry, Multidisciplinary

Liquid Metals: A Novel Possibility of Fabricating 2D Metal Oxides

Shasha Zhao et al.

Summary: Liquid metals have shown great potential in the fabrication of 2D metal oxides due to their solubility, fluidity, reactivity, and ability to act as a symmetric matched substrate for growing high-quality materials. Their unique features make them promising candidates for the further development of 2DMOs.

ADVANCED MATERIALS (2021)

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Article Materials Science, Ceramics

Sturdy memristive switching characteristics of flexible 2D SnO prepared by liquid-to-solid exfoliation

Dong Jin Lee et al.

Summary: Monolayer-thick 2D tin monoxide (SnO) was synthesized by liquid-to-solid exfoliation, showing promise for future flexible nanoelectronics.

CERAMICS INTERNATIONAL (2021)

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Article Materials Science, Multidisciplinary

Emerging 2D metal oxides and their applications

Partha Kumbhakar et al.

Summary: This paper summarizes the research progress on two-dimensional materials over the past decade, focusing on the characteristics and potential applications of two-dimensional metal oxides, as well as comparisons with traditional oxides.

MATERIALS TODAY (2021)

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Review Chemistry, Multidisciplinary

Interfacial Engineering of Room Temperature Liquid Metals

Jun-Heng Fu et al.

Summary: Room temperature liquid metals, particularly gallium-based alloys, exhibit fascinating characteristics derived from both metallic and fluidic natures. Understanding the interfacial effects of liquid metal on diverse surfaces is crucial for explaining fundamental phenomena and enabling applications in unconventional chemical synthesis, energy conversion, and printed electronics. Systematic interpretation of these interfacial issues is essential for developing advanced technologies in RTLMs.

ADVANCED MATERIALS INTERFACES (2021)

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Article Materials Science, Multidisciplinary

Bismuth telluride topological insulator synthesized using liquid metal alloys: Test of NO2 selective sensing

Maedehsadat Mousavi et al.

Summary: By utilizing liquid metal interfaces as reaction media with their autogenous surface potential, highly crystalline bismuth telluride nanostructures were successfully synthesized. Sensors fabricated using these materials exhibit good selectivity and sensitivity for nitrogen dioxide adsorption at low temperatures.

APPLIED MATERIALS TODAY (2021)

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Article Engineering, Electrical & Electronic

The performance limits of hexagonal boron nitride as an insulator for scaled CMOS devices based on two-dimensional materials

Theresia Knobloch et al.

Summary: This article assesses the material parameters and performance limits of hexagonal boron nitride (hBN) as a gate insulator, comparing experimental and theoretical tunnel currents through ultrathin layers of hBN and other 2D gate insulators. Despite its candidacy for many applications in 2D nanoelectronics, excessive leakage currents indicate that hBN is unlikely to be suitable for use as a gate insulator in ultrascaled CMOS devices.

NATURE ELECTRONICS (2021)

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Article Chemistry, Physical

Two-dimensional oxide derived from high-temperature liquid metals via bubble templating

Zheng Hu et al.

Summary: Continuous production of two-dimensional oxides can be achieved by bubbling oxygen into liquid metals with proper choice of dispersion solvents. The use of liquid tin in the bubbling protocol for the first time resulted in high-performance 2D tin oxide obtained in molten salts. The molten-salt based protocol can be explored for the synthesis of a library of functional 2D oxides.

NANO RESEARCH (2021)

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Article Engineering, Electrical & Electronic

High-mobility p-type semiconducting two-dimensional β-TeO2

Ali Zavabeti et al.

Summary: Bilayer beta tellurium dioxide nanosheets were successfully synthesized through surface oxidation of tellurium and selenium mixture, demonstrating high-mobility p-type semiconductor properties. These nanosheets have potential applications in transistor fabrication, showing p-type switching with a high on/off ratio and field-effect hole mobility of up to 232 cm(2) V-1 s(-1) at room temperature. The carrier mobility reached even higher values of 6,000 cm(2) V-1 s(-1) on cooling to -50 degrees C, indicating promising prospects for high-speed and energy-efficient transparent electronics.

NATURE ELECTRONICS (2021)

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Article Nanoscience & Nanotechnology

Gas-mediated liquid metal printing toward large-scale 2D semiconductors and ultraviolet photodetector

Qian Li et al.

Summary: This study presents a gas-mediated fabrication method for centimeter-scale 2D semiconductors and ultraviolet photodetectors using liquid metal-based printing. The research demonstrates the feasibility of directly printing various large-scale 2D materials at ambient air, providing a fast, generic, clean, and scalable technique for manufacturing 2D semiconductors. By exploring the electrical properties and developing low-cost processes, the study successfully creates high-performance fully printed Ga2O3/Si heterojunction photodetectors with excellent sensibility and rapid photoresponse times, offering a feasible approach for mass production of high-performance ultraviolet photodetectors and suggesting a promising direction for large-scale 2D photoelectronic and electronic systems in the future.

NPJ 2D MATERIALS AND APPLICATIONS (2021)

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Article Nanoscience & Nanotechnology

Low Deposition Temperature Amorphous ALD-Ga2O3 Thin Films and Decoration with MoS2 Multilayers toward Flexible Solar-Blind Photodetectors

Yan Yang et al.

Summary: Flexible sensors and photodetectors are important strategies for advanced devices, and the use of amorphous ALD-Ga2O3 thin films has shown promise in fabricating flexible solar-blind photodetectors (SBPDs). Decorating the ALD-Ga2O3 channels with MoS2 multilayers has been found to improve the photocurrent of SBPDs working in the deep ultraviolet region.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

A Liquid Metal Mediated Metallic Coating for Antimicrobial and Antiviral Fabrics

Ki Yoon Kwon et al.

Summary: A new fabric coating technology utilizing liquid metal particles to eradicate pathogens has proven to be highly effective in eliminating over 99% of bacteria, fungi, and viruses. This method shows promise in creating robust antibacterial, antifungal, and antiviral fabrics and surfaces.

ADVANCED MATERIALS (2021)

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Article Chemistry, Physical

Template Approach to Large-Area Non-layered Ga-Group Two-Dimensional Crystals from Printed Skin of Liquid Gallium

Jing Li et al.

Summary: This study introduces an efficient PDMS printing strategy for controllable preparation and transfer of a large-area non-layered 2D Ga2O3 amorphous layer, and proposes a template-confined reaction to achieve other 2D Ga-group crystals, enabling the fabrication of high-performance and multifunctional electronics.

CHEMISTRY OF MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Surface Tension of the Oxide Skin of Gallium-Based Liquid Metals

Stephan Handschuh-Wang et al.

Summary: This article explores the surface tension of gallium-based alloys, determining it to be independent of substrate surface or liquid metal used. By using gradually attenuated vibrations and the puddle height method, the researchers were able to analyze equilibrium shapes and attribute the similarity of surface tension among different alloys to the composition of the oxide skin. The findings suggest potential application of this method to other liquid metal alloys and systems for modeling, simulation, and optimization processes.

LANGMUIR (2021)

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Article Materials Science, Multidisciplinary

A Visible-Blind Photodetector and Artificial Optoelectronic Synapse Using Liquid-Metal Exfoliated ZnO Nanosheets

Vaishnavi Krishnamurthi et al.

Summary: A liquid metal exfoliation technique was utilized to obtain millimeter-scale ZnO nanosheets with a thickness down to 5 nm, showcasing their potential applications in high-performance electronic and optoelectronic devices.

ADVANCED OPTICAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Precise Regulation of Ga-Based Liquid Metal Oxidation

Dawei Wang et al.

Summary: Liquid metals are non-crystalline solids in the molten state with fundamentally different fluidities and metallicities from solid metals. Gallium, with its low toxicity and high thermal and electrical conductivity, has been proposed as a base material for liquid metal construction. The existence of oxides in liquid metals can provide both benefits and challenges, impacting performance and stability in various applications. Oxidation regulation of liquid metals remains a relatively unexplored area with potential for significant advancements in material design and synthesis.

ACCOUNTS OF MATERIALS RESEARCH (2021)

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Article Chemistry, Multidisciplinary

A Liquid Metal Reaction System for Advanced Material Manufacturing

Mengqi Zeng et al.

Summary: Liquid metal, with unique properties like self-limited growth and good rheological properties, shows great potential in the controllable fabrication of 2D materials and functional composite materials. The research on advanced materials manufacturing on liquid metals is still in its infancy, but offers promising prospects for various applications in energy field and beyond.

ACCOUNTS OF MATERIALS RESEARCH (2021)

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Review Automation & Control Systems

Interfacial Tension Modulation of Liquid Metal via Electrochemical Oxidation

Minyung Song et al.

Summary: Recent studies have shown that electrochemical oxidation can significantly decrease the interfacial tension of liquid metals, from approximately 500 mN m(-1) at 0 V to approximately 0 mN m(-1) at less than 1 V. This reversible and controllable change in tension surpasses what is achievable through conventional electrocapillarity or surfactants. The report aims to introduce beginners to this field, clarify misconceptions, and discuss applications and future challenges related to modulating the interfacial tension of liquid metals.

ADVANCED INTELLIGENT SYSTEMS (2021)

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Review Automation & Control Systems

Surface Modification of Gallium-Based Liquid Metals: Mechanisms and Applications in Biomedical Sensors and Soft Actuators

Ki Yoon Kwon et al.

Summary: Surface modifications to gallium-based liquid metals enable unique applications such as soft biomedical sensors and actuators, providing comfort, mechanical compliance, and stretchability.

ADVANCED INTELLIGENT SYSTEMS (2021)

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Article Materials Science, Multidisciplinary

Ultrathin oxysulfide semiconductors from liquid metal: a wet chemical approach

Chung Kim Nguyen et al.

Summary: Metal oxychalcogenides, especially 2D oxysulfide materials, are showing promise in next-generation electronic and optoelectronic devices. A new synthesis approach has been developed to fabricate atomically thin and large-area indium oxysulfide nanosheets with significantly enhanced electronic and optical properties. This method can also be applied to obtain other 2D oxysulfide semiconductors, providing a furnace-free fabrication route.

JOURNAL OF MATERIALS CHEMISTRY C (2021)

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Review Chemistry, Inorganic & Nuclear

An exploration into two-dimensional metal oxides, and other 2D materials, synthesised via liquid metal printing and transfer techniques

Abigail Goff et al.

Summary: The new liquid metal-based technique combines top-down and bottom-up processes to synthesize 2D metal oxides, which can be exfoliated into 2D flakes for use in electronic devices and chemical reactions.

DALTON TRANSACTIONS (2021)

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Review Chemistry, Multidisciplinary

Wide Band Gap Chalcogenide Semiconductors

Rachel Woods-Robinson et al.

CHEMICAL REVIEWS (2020)

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Universal mechanical exfoliation of large-area 2D crystals

Yuan Huang et al.

NATURE COMMUNICATIONS (2020)

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Review Chemistry, Multidisciplinary

Metal Oxysulfides: From Bulk Compounds to Nanomaterials

Clement Larquet et al.

FRONTIERS IN CHEMISTRY (2020)

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Two-Dimensional Amorphous SnOx from Liquid Metal: Mass Production, Phase Transfer, and Electrocatalytic CO2 Reduction toward Formic Acid

Tingbiao Yuan et al.

NANO LETTERS (2020)

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Article Materials Science, Multidisciplinary

Synthesis and Characterization of Large-Area Nanometer-Thin beta-Ga2O3 Films from Oxide Printing of Liquid Metal Gallium

Jacqueline Cooke et al.

PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE (2020)

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Article Materials Science, Multidisciplinary

Liquid metal Ga-Sn alloy based ferrofluids with amorphous nano-sized Fe-Co-B magnetic particles

Chuncheng Yang et al.

JOURNAL OF MATERIALS SCIENCE (2020)

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Design and Integration of a Layered MoS2/GaN van der Waals Heterostructure for Wide Spectral Detection and Enhanced Photoresponse

Xinglai Zhang et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Chemistry, Physical

Complexity and Opportunities in Liquid Metal Surface Oxides

Andrew Martin et al.

CHEMISTRY OF MATERIALS (2020)

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Liquid metal-based synthesis of high performance monolayer SnS piezoelectric nanogenerators

Hareem Khan et al.

NATURE COMMUNICATIONS (2020)

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Nanostructured Tungsten Oxysulfide as an Efficient Electrocatalyst for Hydrogen Evolution Reaction

Prasad Sarma et al.

ACS CATALYSIS (2020)

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Oxidation of Gallium-based Liquid Metal Alloys by Water

Megan A. Creighton et al.

LANGMUIR (2020)

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Two-Step Synthesis of Large-Area 2D Bi2S3Nanosheets Featuring High In-Plane Anisotropy

Kibret A. Messalea et al.

ADVANCED MATERIALS INTERFACES (2020)

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Review Materials Science, Multidisciplinary

Surface Chemistry of Gallium-Based Liquid Metals

Yiran Ding et al.

MATTER (2020)

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Liquid Metals in Catalysis for Energy Applications

Karma Zuraiqi et al.

JOULE (2020)

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Ising ferromagnetism and robust half-metallicity in two-dimensional honeycomb-kagome Cr2O3 layer

Arqum Hashmi et al.

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Ultra-thin lead oxide piezoelectric layers for reduced environmental contamination using a liquid metal-based process

Mohammad B. Ghasemian et al.

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Performance improvement of amorphous Ga 2 O 3 ultraviolet photodetector by annealing under oxygen atmosphere

Changqi Zhou et al.

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Atomically thin TiO2 nanosheets synthesized using liquid metal chemistry

Turki Alkathiri et al.

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Ordered-vacancy-enabled indium sulphide printed in wafer-scale with enhanced electron mobility

Azmira Jannat et al.

MATERIALS HORIZONS (2020)

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Flexible two-dimensional indium tin oxide fabricated using a liquid metal printing technique

Robi S. Datta et al.

NATURE ELECTRONICS (2020)

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Synthesis of 2D cobalt oxide nanosheets using a room temperature liquid metal

Jessica Crawford et al.

RSC ADVANCES (2020)

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2D SnO/In2O3 van der Waals Heterostructure Photodetector Based on Printed Oxide Skin of Liquid Metals

Manal M. Y. A. Alsaif et al.

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Printing of Quasi-2D Semiconducting β-Ga2O3 in Constructing Electronic Devices via Room-Temperature Liquid Metal Oxide Skin

Ju Lin et al.

PHYSICA STATUS SOLIDI-RAPID RESEARCH LETTERS (2019)

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Self-Limiting Galvanic Growth of MnO2 Monolayers on a Liquid Metal-Applied to Photocatalysis

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Epitaxial growth and characterization of high quality In2O3 films on a-plane sapphire substrates by MOCVD

Xuejian Du et al.

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2D materials for quantum information science

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Giant valley splitting in monolayer WS2 by magnetic proximity effect

Tenzin Norden et al.

NATURE COMMUNICATIONS (2019)

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Wafer-Sized Ultrathin Gallium and Indium Nitride Nanosheets through the Ammonolysis of Liquid Metal Derived Oxides

Nitu Syed et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Atomically Thin 2D Transition Metal Oxides: Structural Reconstruction, Interaction with Substrates, and Potential Applications

Tong Yang et al.

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Atomically Thin Ga2S3 from Skin of Liquid Metals for Electrical, Optical, and Sensing Applications

Manal M. Y. A. Alsaif et al.

ACS APPLIED NANO MATERIALS (2019)

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Brushed Crystallized Ultrathin Oxides: Recrystallization and Deep-Ultraviolet Imaging Application

Richeng Lin et al.

ACS APPLIED ELECTRONIC MATERIALS (2019)

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Control of Gallium Oxide Growth on Liquid Metal Eutectic Gallium/Indium Nanoparticles via Thiolation

Zachary J. Farrell et al.

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Metallic Bond-Enabled Wetting Behavior at the Liquid Ga/CuGa2 Interfaces

Yuntao Cui et al.

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Highly Sensitive and Wearable In2O3 Nanoribbon Transistor Biosensors with Integrated On-Chip Gate for Glucose Monitoring in Body Fluids

Qingzhou Liu et al.

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Evolution of 2D tin oxides on the surface of molten tin

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CHEMICAL COMMUNICATIONS (2018)

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Liquid metals: fundamentals and applications in chemistry

T. Daeneke et al.

CHEMICAL SOCIETY REVIEWS (2018)

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Review Chemistry, Multidisciplinary

Recent progress in the assembly of nanodevices and van der Waals heterostructures by deterministic placement of 2D materials

Riccardo Frisenda et al.

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Room Temperature Electrochemical Synthesis of Crystalline GaOOH Nanoparticles from Expanding Liquid Metals

Benchaporn Lertanantawong et al.

LANGMUIR (2018)

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Bi2O3 monolayers from elemental liquid bismuth

Kibret A. Messalea et al.

NANOSCALE (2018)

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Ultrathin tellurium dioxide: emerging direct bandgap semiconductor with high-mobility transport anisotropy

Shiying Guo et al.

NANOSCALE (2018)

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Printing two-dimensional gallium phosphate out of liquid metal

Nitu Syed et al.

NATURE COMMUNICATIONS (2018)

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Growth of 2D GaN Single Crystals on Liquid Metals

Yunxu Chen et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2018)

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Synthesis of 2D transition metal dichalcogenides by chemical vapor deposition with controlled layer number and morphology

Jiawen You et al.

NANO CONVERGENCE (2018)

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Engineering Valence Band Dispersion for High Mobility p-Type Semiconductors

Benjamin A. D. Williamson et al.

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A liquid metal reaction environment for the room-temperature synthesis of atomically thin metal oxides

Ali Zavabeti et al.

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Metal-based magnetic fluids with core-shell structure FeB@SiO2 amorphous particles

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Shape-transformable liquid metal nanoparticles in aqueous solution

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Wafer-scale two-dimensional semiconductors from printed oxide skin of liquid metals

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Giant magnetic splitting inducing near-unity valley polarization in van der Waals heterostructures

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Wafer-Scale Synthesis of Semiconducting SnO Monolayers from Interfacial Oxide Layers of Metallic Liquid Tin

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Stretchable and Soft Electronics using Liquid Metals

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Tuning two-dimensional nanomaterials by intercalation: materials, properties and applications

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2D layered group IIIA metal chalcogenides: synthesis, properties and applications in electronics and optoelectronics

Wenjuan Huang et al.

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2D materials and van der Waals heterostructures

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Ionic imbalance induced self-propulsion of liquid metals

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2D Tin Monoxide-An Unexplored p-Type van der Waals Semiconductor: Material Characteristics and Field Effect Transistors

Kachirayil J. Saji et al.

ADVANCED ELECTRONIC MATERIALS (2016)

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Review Nanoscience & Nanotechnology

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