期刊
CHEMICAL REVIEWS
卷 122, 期 2, 页码 1543-1625出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.chemrev.1c00403
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资金
- National Institute of Health [GM120281]
- National Science Foundation [CHE-1955663]
- Welch Foundation [AT-0041]
- Eugene McDermott Graduate Fellowship, UT Dallas
Visible light-induced transition metal catalysis has emerged as an important development in organic photocatalysis, leading to unprecedented transformations and improvements of known reactions. This method utilizes a single catalytic cycle to harness photon energy, and synergistically combines catalyst-substrate interaction with photoinduced processes.
In recent years, visible light-induced transition metal catalysis has emerged as a new paradigm in organic photocatalysis, which has led to the discovery of unprecedented transformations as well as the improvement of known reactions. In this subfield of photocatalysis, a transition metal complex serves a double duty by harvesting photon energy and then enabling bond forming/breaking events mostly via a single catalytic cycle, thus contrasting the established dual photocatalysis in which an exogenous photosensitizer is employed. In addition, this approach often synergistically combines catalyst-substrate interaction with photoinduced process, a feature that is uncommon in conventional photoredox chemistry. This Review describes the early development and recent advances of this emerging field.
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