4.6 Article

Numerical simulation of multiphase flow in a full coal-direct chemical looping combustion process

期刊

CHEMICAL ENGINEERING SCIENCE
卷 248, 期 -, 页码 -

出版社

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.ces.2021.117233

关键词

Chemical looping combustion; Gas-solid flow; Fluidized bed; Reactor optimization; Numerical simulation

资金

  1. Australian Research Council [DP180101232, FT190100361]

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This study used a multi-fluid model to investigate the gas-solid hydrodynamics in a CDCL combustion unit, revealing that the solid circulation rate is controlled by the gas flow rate, higher combustor gas velocity reduces system pressure, and increased L-valve gas velocity affects local pressure.
Chemical looping combustion (CLC) is a promising clean combustion technology alternative to conventional oxy-combustion, yet the full loop flow details are not well understood. In this work, a multi fluid model based on the Eulerian-Eulerian framework is used to study the gas-solid hydrodynamics in a full-loop Coal-direct chemical looping (CDCL) combustion unit with a unique moving-bed fuel reactor. The unique fluidization states are described throughout the full-loop system. Then, the influences of several operating conditions on the solid circulation rate and pressure distribution are investigated. It is shown that the solids circulation rate is dominantly controlled by the gas flow rate on the standpipe of the L-valve. Meanwhile, a higher combustor gas velocity reduces the pressure of the whole system and an increased L-valve gas velocity influences the pressure distribution slightly but increases the local pressure at the L-valve. This work provides a cost-effective tool for understanding and optimizing the CDCL process. (c) 2021 Elsevier Ltd. All rights reserved.

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