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Advances in allylic and benzylic C-H bond functionalization enabled by metallaphotoredox catalysis

期刊

CHEMICAL COMMUNICATIONS
卷 58, 期 2, 页码 171-184

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ROYAL SOC CHEMISTRY
DOI: 10.1039/d1cc06285a

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  1. King Abdullah University of Science and Technology (KAUST), Saudi Arabia, Office of Sponsored Research [URF/1/4384]

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Metallaphoto-catalysis is an efficient platform for constructing various chemical bonds, with the transformation of native functionalities such as C(sp(3))-H bonds into functional molecules being an attractive strategy in organic synthesis. The merging of two powerful methodologies, metallaphoto-catalyzed benzylic and allylic C(sp(3))-H bond functionalizations, offers general and mild approaches for diversifying alkylbenzenes and alkenes.
Metallaphoto-catalysis has been established as a robust platform for efficient construction of a range of chemical bonds. Moreover, transformation of native functionalities such as C(sp(3))-H bonds to produce functional molecules represents one of the most attractive strategies in organic synthesis. Merging two powerful methodologies, metallaphoto-catalyzed benzylic and allylic C(sp(3))-H bond functionalizations provide a series of general and mild approaches for diversification of alkylbenzenes and alkenes.

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