期刊
CARBON
卷 184, 期 -, 页码 526-533出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.carbon.2021.08.061
关键词
Graphdiyne; Magnetoresistance; Magnetotransport; Weak localization; Magnetic polaron model
资金
- Natural Science Foundations of Fujian Province [2020J01196, 2020J01193]
- Fujian Natural Science Foundation for Distinguished Young Scholars [2020J06042]
- Cultivation plan of outstanding young scientific research talents of Fujian Education Department [J1-1323]
This study developed a modified non-transferred graphdiyne film synthesis method and investigated its magnetoresistance effect. A temperature-dependent crossover between positive and negative magnetoresistance was observed in the graphdiyne film, with mechanisms involving the magnetic polaron model and weak localization.
Two-dimensional layered carbon materials such as graphene constructed by sp(2) hybridization have raised considerable interest due to their large, non-saturating magnetoresistance. As a new sp-sp(2) hybridization structure layered carbon material, the transport performance of graphdiyne has been founded comparable with graphene, while the magnetoresistance remains to be clarified. In this work, we developed a modified non-transferred graphdiyne film synthesized method and studied its magnetoresistance effect. We observed an unexpected temperature-dependent crossover between positive and negative magnetoresistance in graphdiyne film. The film shows negative magnetoresistance at 5-19 K, the maximum intensity of the negative magnetoresistance was about 150% at 5 K under 3 T magnetic field. It presents positive magnetoresistance at 19-21 K under 3 T magnetic field, the magnetoresistance value reached 150% at 20 K. The mechanism of crossover positive and negative magnetoresistance originates from a superposition of the magnetic polaron model and weak localization. (C) 2021 Published by Elsevier Ltd.
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