Interfacial Fe-O-Ni-O-Fe Bonding Regulates the Active Ni Sites of Ni-MOFs via Iron Doping and Decorating with FeOOH for Super-Efficient Oxygen Evolution

Article Chemistry, Multidisciplinary

Spectroscopic and Electrokinetic Evidence for a Bifunctional Mechanism of the Oxygen Evolution Reaction**

Lichen Bai et al.

Summary: The study experimentally validated two different mechanisms for oxygen evolution reaction catalysts: one is a bifunctional mechanism, and the other is a conventional four-step proton-coupled electron transfer mechanism.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Facile Synthesis of Two-Dimensional Iron/Cobalt Metal-Organic Framework for Efficient Oxygen Evolution Electrocatalysis

Kai Ge et al.

Summary: A facile synthesis method was reported for the preparation of two-dimensional bimetallic metal-organic frameworks with excellent electrocatalytic activity for the oxygen evolution reaction. Experimental and theoretical studies revealed that the morphology and co-doping of Fe/Co played crucial roles in enhancing the electrocatalytic performance of the material. The simple and efficient synthetic approach is promising for the mass production and future commercialization of functional two-dimensional MOFs with low cost and high yield.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Surface-Adsorbed Carboxylate Ligands on Layered Double Hydroxides/Metal-Organic Frameworks Promote the Electrocatalytic Oxygen Evolution Reaction

Cheng-Fei Li et al.

Summary: The study revealed the extraordinary role and mechanism of carboxylate ligands on bimetallic/tri-metallic layered double hydroxides/MOFs catalytic activity for the oxygen evolution reaction, enhancing the electrocatalytic performance of OER.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Trimetallic Spinel NiCo2-xFexO4 Nanoboxes for Highly Efficient Electrocatalytic Oxygen Evolution

Yi Huang et al.

Summary: The study successfully designed and synthesized optimized porous Co-based trimetallic spinel oxide nanoboxes with superior electrocatalytic performance for the oxygen evolution reaction. The structural and compositional advantages enable the nanoboxes to exhibit excellent performance in alkaline electrolyte.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Short-Range Ordered Iridium Single Atoms Integrated into Cobalt Oxide Spinel Structure for Highly Efficient Electrocatalytic Water Oxidation

Jieqiong Shan et al.

Summary: This study proposes a method to integrate noble metal atoms into the lattice of transition metal oxides to create a new type of hybrid structure, showing that iridium single atoms can be effectively accommodated into cobalt spinel oxide. The resultant catalyst exhibits significantly higher electrocatalytic activity under acidic conditions, with improved corrosion resistance and oxidative potentials. This work eliminates the close-packing limitation of noble metals and offers promising opportunities for creating analogues with desired topologies for various catalytic applications.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Multidisciplinary

Interfacial Electron Engineering of Palladium and Molybdenum Carbide for Highly Efficient Oxygen Reduction

Liang Huang et al.

Summary: The study demonstrates the fabrication of Mo2C-coupled Pd atomic layers heterostructure electrocatalyst through precise control of metal-organic framework confinement and covalent interaction. The resulting AL-Pd/Mo2C showed the highest ORR electrochemical activity and stability, significantly outperforming traditional Pt/C, Pd/C, and Pd nanoparticles catalysts.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Multidisciplinary

Electronic Modulation Caused by Interfacial Ni-O-M (M=Ru, Ir, Pd) Bonding for Accelerating Hydrogen Evolution Kinetics

Liming Deng et al.

Summary: Designing a well-defined metal-support interfacial bond is an effective strategy to optimize the intrinsic activity of noble metals, but it is also challenging. The developed quantum-sized metal nanoparticles anchored on nickel metal-organic framework nanohybrids demonstrate excellent hydrogen evolution reaction (HER) activity at all pH values, surpassing even commercial Pt/C and recent noble-metal catalysts. The interfacial-bond-induced electron redistribution plays a crucial role in enhancing the reaction kinetics and overall performance of the hybrids.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Interfacial Engineering of W2N/WC Heterostructures Derived from Solid-State Synthesis: A Highly Efficient Trifunctional Electrocatalyst for ORR, OER, and HER

Jinxiang Diao et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Autologous Cobalt Phosphates with Modulated Coordination Sites for Electrocatalytic Water Oxidation

Jing Qi et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Inorganic & Nuclear

Cobalt-Based MOF-on-MOF Two-Dimensional Heterojunction Nanostructures for Enhanced Oxygen Evolution Reaction Electrocatalytic Activity

Qingqing Zha et al.

INORGANIC CHEMISTRY (2020)

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Review Chemistry, Physical

Metal-Organic Framework-Based Materials for Energy Conversion and Storage

Tianjie Qiu et al.

ACS ENERGY LETTERS (2020)

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Article Chemistry, Physical

Hierarchical trimetallic layered double hydroxide nanosheets derived from 2D metal-organic frameworks for enhanced oxygen evolution reaction

Wen-Da Zhang et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Chemistry, Multidisciplinary

NiMn-Based Bimetal-Organic Framework Nanosheets Supported on Multi-Channel Carbon Fibers for Efficient Oxygen Electrocatalysis

Weiren Cheng et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Multidisciplinary Sciences

Boosting Lattice Oxygen Oxidation of Perovskite to Efficiently Catalyze Oxygen Evolution Reaction by FeOOH Decoration

Jia-Wei Zhao et al.

RESEARCH (2020)

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Article Chemistry, Multidisciplinary

Strong Electronic Interaction Enhanced Electrocatalysis of Metal Sulfide Clusters Embedded Metal-Organic Framework Ultrathin Nanosheets toward Highly Efficient Overall Water Splitting

Ming Zhao et al.

ADVANCED SCIENCE (2020)

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Article Chemistry, Multidisciplinary

Bimetal-organic framework MIL-53(Co-Fe): an efficient and robust electrocatalyst for the oxygen evolution reaction

Maowen Xie et al.

NANOSCALE (2020)

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Review Chemistry, Multidisciplinary

Structural Design and Electronic Modulation of Transition-Metal-Carbide Electrocatalysts toward Efficient Hydrogen Evolution

Qingsheng Gao et al.

ADVANCED MATERIALS (2019)

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Article Chemistry, Multidisciplinary

Highly Conductive Bimetallic Ni-Fe Metal Organic Framework as a Novel Electrocatalyst for Water Oxidation

Fuqin Zheng et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2019)

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Article Chemistry, Multidisciplinary

A Surfactant-Free and Scalable General Strategy for Synthesizing Ultrathin Two-Dimensional Metal-Organic Framework Nanosheets for the Oxygen Evolution Reaction

Linzhou Zhuang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Chemistry, Physical

In-situ Growth of a Bimetallic Cobalt-Nickel Organic Framework on Iron Foam: Achieving the Electron Modification on a Robust Self-supported Oxygen Evolution Electrode

Pei Luo et al.

CHEMCATCHEM (2019)

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Article Multidisciplinary Sciences

Boosting oxygen evolution of single-atomic ruthenium through electronic coupling with cobalt-iron layered double hydroxides

Pengsong Li et al.

NATURE COMMUNICATIONS (2019)

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Article Chemistry, Multidisciplinary

Layered Structure Causes Bulk NiFe Layered Double Hydroxide Unstable in Alkaline Oxygen Evolution Reaction

Rong Chen et al.

ADVANCED MATERIALS (2019)

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Article Multidisciplinary Sciences

A bio-inspired coordination polymer as outstanding water oxidation catalyst via second coordination sphere engineering

Wenlong Li et al.

NATURE COMMUNICATIONS (2019)

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Article Chemistry, Multidisciplinary

A General Method to Ultrathin Bimetal-MOF Nanosheets Arrays via In Situ Transformation of Layered Double Hydroxides Arrays

Bingqing Wang et al.

SMALL (2019)

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Article Chemistry, Physical

Low-Crystalline Bimetallic Metal-Organic Framework Electrocatalysts with Rich Active Sites for Oxygen Evolution

Jiantao Li et al.

ACS ENERGY LETTERS (2019)

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Article Chemistry, Physical

Defective metal-organic framework derivative by room-temperature exfoliation and reduction for highly efficient oxygen evolution reaction

Zehua Zou et al.

JOURNAL OF MATERIALS CHEMISTRY A (2019)

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Article Chemistry, Multidisciplinary

Iron carbonate hydroxide templated binary metal-organic frameworks for highly efficient electrochemical water oxidation

Jian Du et al.

CHEMICAL COMMUNICATIONS (2019)

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Article Chemistry, Multidisciplinary

In Situ Grown Epitaxial Heterojunction Exhibits High-Performance Electrocatalytic Water Splitting

Changrong Zhu et al.

ADVANCED MATERIALS (2018)

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Article Chemistry, Multidisciplinary

Bifunctional Electrocatalysts for Overall Water Splitting from an Iron/Nickel-Based Bimetallic Metal-Organic Framework/Dicyandiamide Composite

Xiaojia Zhao et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

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Article Chemistry, Multidisciplinary

Electrochemical Exfoliation of Pillared-Layer Metal-Organic Framework to Boost the Oxygen Evolution Reaction

Jin Huang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

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Article Multidisciplinary Sciences

Atomic-level insight into super-efficient electrocatalytic oxygen evolution on iron and vanadium co-doped nickel (oxy)hydroxide

Jian Jiang et al.

NATURE COMMUNICATIONS (2018)

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Article Multidisciplinary Sciences

Systematic design of superaerophobic nanotube-array electrode comprised of transition-metal sulfides for overall water splitting

Haoyi Li et al.

NATURE COMMUNICATIONS (2018)

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Article Chemistry, Physical

Uncovering the mechanisms of electrolyte permeation in porous electrodes for redox flow batteries through real time in situ 3D imaging

Farid Tariq et al.

SUSTAINABLE ENERGY & FUELS (2018)

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Article Chemistry, Physical

Interfacial Interaction between FeOOH and Ni-Fe LDH to Modulate the Local Electronic Structure for Enhanced OER Electrocatalysis

Jiande Chen et al.

ACS CATALYSIS (2018)

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Article Chemistry, Inorganic & Nuclear

Mixed-Metal Strategy on Metal-Organic Frameworks (MOFs) for Functionalities Expansion: Co Substitution Induces Aerobic Oxidation of Cyclohexene over Inactive Ni-MOF-74

Dengrong Sun et al.

INORGANIC CHEMISTRY (2015)

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Article Chemistry, Physical

From the Sabatier principle to a predictive theory of transition-metal heterogeneous catalysis

Andrew J. Medford et al.

JOURNAL OF CATALYSIS (2015)

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Article Chemistry, Physical

Water Reaction Mechanism in Metal Organic Frameworks with Coordinatively Unsaturated Metal Ions: MOF-74

Kui Tan et al.

CHEMISTRY OF MATERIALS (2014)

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Article Chemistry, Multidisciplinary

Amorphous FeOOH Oxygen Evolution Reaction Catalyst for Photoelectrochemical Water Splitting

William D. Chemelewski et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2014)

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Article Chemistry, Multidisciplinary

Rationalization of Interactions in Precious Metal/Ceria Catalysts Using the d-Band Center Model

N. Acerbi et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2013)

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Article Chemistry, Physical

Ion Exchange in Metal-Organic Framework for Water Purification: Insight from Molecular Simulation

Anjaiah Nalaparaju et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2012)

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Article Chemistry, Physical

In Situ Raman Study of Nickel Oxide and Gold-Supported Nickel Oxide Catalysts for the Electrochemical Evolution of Oxygen

Boon Siang Yeo et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2012)

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Article Chemistry, Multidisciplinary

Structure-Activity Correlations in a Nickel-Borate Oxygen Evolution Catalyst

D. Kwabena Bediako et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2012)

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Interfacial Fe-O-Ni-O-Fe Bonding Regulates the Active Ni Sites of Ni-MOFs via Iron Doping and Decorating with FeOOH for Super-Efficient Oxygen Evolution

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