期刊
ADVANCED SYNTHESIS & CATALYSIS
卷 364, 期 1, 页码 158-164出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.202100884
关键词
Aurachins; Suzuki-Miyaura coupling; Prenylated quinolines; Total synthesis; Natural product
资金
- Project DEAL
A polyprenyl side chain was introduced into the heterocyclic quinoline moiety through Suzuki-Miyaura coupling, enabling the synthesis of Aurachin B from Stigmatella aurantiaca. This prenylated quinoline could then be transformed into the related compound Aurachin A through an epoxidation-ring opening cascade.
A polyprenyl side chain could be introduced into the heterocyclic quinoline moiety through Suzuki-Miyaura coupling of the corresponding quinoline-N-oxide with a polyprenyl boronic acid. This tool could be utilized for the synthesis of the natural product Aurachin B from the myxobacterium Stigmatella aurantiaca. This prenylated quinoline could then be transformed into the related Aurachin A through an epoxidation-ring opening cascade.
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