☆ 4.8 Review

Recent Advances in Design of Electrocatalysts for High-Current-Density Water Splitting

ADVANCED MATERIALS (2022)

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Article Chemistry, Physical

Self-supported Pt-CoO networks combining high specific activity with high surface area for oxygen reduction

Gustav W. Sievers et al.

Summary: A new concept of self-supported platinum-cobalt oxide networks has been proposed, combining high specific activity with a high ECSA, promising a stable fuel-cell operation. This concept exceeds the US Department of Energy targets for Pt-related ORR mass activity.

NATURE MATERIALS (2021)

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Article Chemistry, Physical

Synergistic Interaction of Double/Simple Perovskite Heterostructure for Efficient Hydrogen Evolution Reaction at High Current Density

Yingying Liu et al.

Summary: The study introduces a novel catalyst PB0.94C-DSPH prepared using a specific double perovskite precursor, exhibiting excellent performance and long-term stability for hydrogen evolution reaction at high current densities.

SMALL METHODS (2021)

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Article Chemistry, Multidisciplinary

Efficient Hydrogen Evolution of Oxidized Ni-N3 Defective Sites for Alkaline Freshwater and Seawater Electrolysis

Wenjie Zang et al.

Summary: In the study, atomically dispersed Ni with triple nitrogen coordination (Ni-N-3) was shown to achieve efficient hydrogen evolution reaction (HER) performance in alkaline media. These catalysts exhibited overpotentials as low as 102 and 139 mV at 10 mA cm(-2) in alkaline freshwater and seawater electrolytes, respectively, outperforming previously reported results.

ADVANCED MATERIALS (2021)

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Article Electrochemistry

NiCu mixed metal oxide catalyst for alkaline hydrogen evolution in anion exchange membrane water electrolysis

Alaa Y. Faid et al.

Summary: The optimization of nickel-copper catalysts for cathode performance in anion exchange membrane (AEM) water electrolysis has been reported, with NiCu mixed metal oxide nanosheets showing rapid kinetics for the hydrogen evolution reaction (HER). In alkaline electrolytes, the activity and stability of NiCu MMO increase with KOH concentration, and the use of Nafion ionomer in the ink results in higher HER current density. The NiCu MMO cathode, paired with Ir black as the anode, achieves AEM electrolyzer performance comparable to PEM water electrolysis.

ELECTROCHIMICA ACTA (2021)

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Article Chemistry, Multidisciplinary

A Durable and Efficient Electrocatalyst for Saline Water Splitting with Current Density Exceeding 2000 mA cm-2

Fengning Yang et al.

Summary: Water electrolysis is a promising method for industrial hydrogen production to achieve a sustainable and green hydrogen economy, but high technology costs limit market share. Developing efficient and economical electrocatalysts is crucial for cost reduction. Electrolysis in seawater electrolyte can further reduce feedstock costs.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Stable and Highly Efficient Hydrogen Evolution from Seawater Enabled by an Unsaturated Nickel Surface Nitride

Huanyu Jin et al.

Summary: A novel unsaturated nickel surface nitride catalyst has been developed for efficient and stable hydrogen electrocatalytic production in alkaline seawater. The catalyst shows lower overpotential compared to traditional metal nitrides and can effectively generate hydronium ions in high-pH electrolyte.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Tip-Enhanced Electric Field: A New Mechanism Promoting Mass Transfer in Oxygen Evolution Reactions

Peng Liu et al.

Summary: In this study, NiFe alloy nanocone arrays were used to enhance the oxygen evolution reaction (OER) rate and outperform state-of-the-art OER electrocatalysts. The high-curvature tips on the nanocones induce a local electric field that significantly increases the concentration of hydroxide ions near the active sites, promoting OER activity. This local field enhanced OER kinetics is suggested to be a generic effect applicable to other OER catalysts.

ADVANCED MATERIALS (2021)

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Article Multidisciplinary Sciences

A Ta-TaS2 monolith catalyst with robust and metallic interface for superior hydrogen evolution

Qiangmin Yu et al.

Summary: The study presents a mechanically stable monolith electrocatalyst that achieves superior hydrogen evolution at large current densities.

NATURE COMMUNICATIONS (2021)

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Article Chemistry, Multidisciplinary

In Situ Formation of Nano Ni-Co Oxyhydroxide Enables Water Oxidation Electrocatalysts Durable at High Current Densities

Jehad Abed et al.

Summary: A novel synthesis method of nanocrystalline Ni-Co-Se using ball milling at cryogenic temperature is reported, with an anodizing mechanism discovered during OER to enhance the electrocatalyst performance. The resulting electrocatalyst shows sustained performance in various devices, including water electrolyzer and CO2-to-ethylene electrolyzer, achieving record-setting full cell voltage at high current density.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Design of Aligned Porous Carbon Films with Single-Atom Co-N-C Sites for High-Current-Density Hydrogen Generation

Rui Liu et al.

Summary: A carbon film embedded with single-atom Co-N-C sites was designed to achieve exceptional HER performance at high current densities, delivering 500 and 1000 mA cm(-2) in acid with overpotentials of 272 and 343 mV, respectively, and operating stably for at least 32 hours under static conditions. The findings pave the road towards rational design of SACs with improved activity and stability at high current densities in gas-evolving electrocatalytic processes.

ADVANCED MATERIALS (2021)

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Article Engineering, Environmental

Hierarchical nano/micro/macro-assembled integrated electrode with high-performance water electro-oxidation

Tong Liu et al.

Summary: The study presents a hierarchical electrode design with oxygen vacancies, combining nickel foam, copper micro-pillars, and cobalt oxide, providing large surface area and channels for efficient proton and electron transfer. This structure enhances the oxygen catalytic performance and exhibits excellent OER performance at high current densities.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Chemistry, Multidisciplinary

Interfacial sp C-O-Mo Hybridization Originated High-Current Density Hydrogen Evolution

Yuan Yao et al.

Summary: The GDY/MoO3 material demonstrates efficient hydrogen evolution reaction with high-current density through rational design of sp C-O-Mo hybridization, creating new intrinsic catalytic active sites and increasing the amount of active sites. This approach allows for outstanding HER activity in alkaline electrolyte and decent activity and stability in natural seawater.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Multidisciplinary

Cr-Doped CoP Nanorod Arrays as High-Performance Hydrogen Evolution Reaction Catalysts at High Current Density

Lipeng Zhang et al.

Summary: The Cr-doped CoP nanorod arrays on carbon cloth (Cr-CoP-NR/CC) exhibited superior performance as HER catalysts with high stability and efficiency at high current densities, indicating great potential to replace costly Pt-based HER catalysts in water electrolyzers.

SMALL (2021)

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Article Multidisciplinary Sciences

IrW nanochannel support enabling ultrastable electrocatalytic oxygen evolution at 2Acm-2 in acidic media

Rui Li et al.

Summary: This study presents a support-stabilized catalyst for proton exchange membrane electrolyzers, which balances high activity and stability in oxygen evolution reaction. By altering the charge distribution and size of surface clusters, the catalyst achieves both stability and high activity.

NATURE COMMUNICATIONS (2021)

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Article Nanoscience & Nanotechnology

Rational Design of Superior Electrocatalysts for Water Oxidation: Crystalline or Amorphous Structure?

Daqin Guan et al.

Summary: This article analyzes the origins of changes in crystalline, amorphous, and crystalline-amorphous materials during/after the OER in water splitting, discusses the potential effects on catalyst activity and stability based on recent representative studies, aiming to guide future OER catalyst design.

SMALL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Stabilized hydroxide-mediated nickel-based electrocatalysts for high-current-density hydrogen evolution in alkaline media

Yuting Luo et al.

Summary: This study presents a nickel-based electrocatalyst mediated by hydroxide for high-current-density hydrogen evolution, showing excellent stability and efficiency. By controlling the charge redistribution of nickel sites and introducing iron elements, it can promote the water dissociation step at high current densities, enhancing the catalytic activity.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Article Nanoscience & Nanotechnology

Enhancing Hydrogen Evolution Electrocatalytic Performance in Neutral Media via Nitrogen and Iron Phosphide Interactions

Siyu Zhao et al.

Summary: A new material, grapevine-shaped N-doped iron phosphide on carbon nanotubes, has been developed as an efficient HER catalyst in neutral media. The optimized catalyst shows a lower overpotential compared to a commercial catalyst at a high current density, indicating its excellent performance. The study demonstrates that the interaction between nitrogen and iron phosphides can enhance the active structures and stabilize metal phosphide electrocatalysts for HER.

SMALL SCIENCE (2021)

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Article Nanoscience & Nanotechnology

Dynamic Surface Chemistry of Catalysts in Oxygen Evolution Reaction

Zongkui Kou et al.

Summary: The dynamic surface chemistry of OER electrocatalysts is influenced by various factors, including the nature of catalysts/precatalysts, reaction and service conditions, and external fields. Due to the local, time-dependent and instant nature, there are considerable challenges in tracing, modelling and understanding the complete dynamic surface chemistry of catalysts in OER. Computational studies and dynamic simulations help provide key insights and there is a critical need for a multiscale computational modelling approach encompassing all these aspects.

SMALL SCIENCE (2021)

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Article Chemistry, Physical

On the effect of anion exchange ionomer binders in bipolar electrode membrane interface water electrolysis

Britta Mayerhoefer et al.

Summary: Bipolar membrane|electrode interface water electrolyzers (BPEMWE) show superior performance compared to proton exchange membrane (PEM) water electrolyzers, primarily due to reduced contact resistances stemming from adhesive effects between oppositely charged polymers. The study indicates that the local pH at a metal surface is strongly correlated with the pH of the surrounding solution rather than the type of ionomer used.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Nanoscience & Nanotechnology

Manipulating Electrocatalysis using Mosaic Catalysts

Yuting Luo et al.

Summary: Researchers have developed a mosaic catalyst that has shown significant success in enhancing catalytic activity. By enhancing mass transferability and local electric field strength, the catalytic performance of the mosaic catalysts is significantly improved.

SMALL SCIENCE (2021)

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Article Nanoscience & Nanotechnology

Beyond Platinum: Defects Abundant CoP3/Ni2P Heterostructure for Hydrogen Evolution Electrocatalysis

Lijie Zhang et al.

Summary: This study introduces a method to enhance the hydrogen evolution reaction activity by introducing vacancy defects at the interface of CoP3/Ni2P heterostructure, showing superior catalytic performance compared to commercial Pt/C.

SMALL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Topological Engineering of Pt-Group-Metal-Based Chiral Crystals toward High-Efficiency Hydrogen Evolution Catalysts

Qun Yang et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Advanced Bifunctional Oxygen Reduction and Evolution Electrocatalyst Derived from Surface-Mounted Metal-Organic Frameworks

Weijin Li et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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CO2 electrolysis to multicarbon products at activities greater than 1 A cm-2

F. Pelayo Garcia de Arquer et al.

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Accelerated Dinitrogen Electroreduction to Ammonia via Interfacial Polarization Triggered by Single-Atom Protrusions

Jie Li et al.

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In-situ structure and catalytic mechanism of NiFe and CoFe layered double hydroxides during oxygen evolution

Fabio Dionigi et al.

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Boosting Activity on Co4N Porous Nanosheet by Coupling CeO2for Efficient Electrochemical Overall Water Splitting at High Current Densities

Hongming Sun et al.

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Canonic-Like HER Activity of Cr1-xMoxB2 Solid Solution: Overpowering Pt/C at High Current Density

Hyounmyung Park et al.

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Selective Loading of Atomic Platinum on a RuCeOxSupport Enables Stable Hydrogen Evolution at High Current Densities

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Favorable Amorphous-Crystalline Iron Oxyhydroxide Phase Boundaries for Boosted Alkaline Water Oxidation

Yanling Qiu et al.

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Cobalt phosphide nanoarrays with crystalline-amorphous hybrid phase for hydrogen production in universal-pH

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Spontaneously separated intermetallic Co3Mo from nanoporous copper as versatile electrocatalysts for highly efficient water splitting

Hang Shi et al.

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High-throughput production of cheap mineral-based two-dimensional electrocatalysts for high-current-density hydrogen evolution

Chi Zhang et al.

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Boosting hydrogen evolution on MoS2 via co-confining selenium in surface and cobalt in inner layer

Zhilong Zheng et al.

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2D CoOOH Sheet-Encapsulated Ni2P into Tubular Arrays Realizing 1000 mA cm-2-Level-Current-Density Hydrogen Evolution Over 100 h in Neutral Water

Shucong Zhang et al.

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Water electrolysers with closed and open electrochemical systems

Marie Francine Lagadec et al.

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Fabrication of a Robust PEM Water Electrolyzer Based on Non-Noble Metal Cathode Catalyst: [Mo3S13]2- Clusters Anchored to N-Doped Carbon Nanotubes

Peter K. R. Holzapfel et al.

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Periodic Porous 3D Electrodes Mitigate Gas Bubble Traffic during Alkaline Water Electrolysis at High Current Densities

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High-Efficiency Anion Exchange Membrane Water Electrolysis Employing Non-Noble Metal Catalysts

Pengzuo Chen et al.

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Superior performance of anion exchange membrane water electrolyzer: Ensemble of producing oxygen vacancies and controlling mass transfer resistance

Yoo Sei Park et al.

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Key role of chemistry versus bias in electrocatalytic oxygen evolution

Hong Nhan Nong et al.

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CFD Modeling and Experimental Validation of an Alkaline Water Electrolysis Cell for Hydrogen Production

Jesus Rodriguez et al.

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Jason K. Lee et al.

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Microkinetic model for pH- and potential-dependent oxygen evolution during water splitting on Fe-doped β-NiOOH

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Ultrafine oxygen-defective iridium oxide nanoclusters for efficient and durable water oxidation at high current densities in acidic media

Zhipeng Yu et al.

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Simultaneous interfacial chemistry and inner Helmholtz plane regulation for superior alkaline hydrogen evolution

Bao Zhang et al.

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High performance multicomponent bifunctional catalysts for overall water splitting

Ranjith Bose et al.

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In Situ Growth of Ru Nanoparticles on (Fe,Ni)(OH)2 to Boost Hydrogen Evolution Activity at High Current Density in Alkaline Media

Xin Xiao et al.

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Exceptional performance of hierarchical Ni-Fe oxyhydroxide@NiFe alloy nanowire array electrocatalysts for large current density water splitting

Caiwu Liang et al.

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Unveiling the Layer-Dependent Catalytic Activity of PtSe2 Atomic Crystals for the Hydrogen Evolution Reaction

Dake Hu et al.

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Yoonseok Choi et al.

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Superaerophobic Nickel Phosphide Nanoarray Catalyst for Efficient Hydrogen Evolution at Ultrahigh Current Densities

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Se-Doping Activates FeOOH for Cost-Effective and Efficient Electrochemical Water Oxidation

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Double-Site Ni-W Nanosheet for Best Alkaline HER Performance at High Current Density >500 mA cm-2

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Atomically dispersed platinum supported on curved carbon supports for efficient electrocatalytic hydrogen evolution

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Ultrahigh-current-density niobium disulfide catalysts for hydrogen evolution

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Morphological and Electronic Tuning of Ni2P through Iron Doping toward Highly Efficient Water Splitting

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Improving electrocatalytic activity of iridium for hydrogen evolution at high current densities above 1000 mA cm-2

Peng Jiang et al.

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Morphology and surface chemistry engineering toward pH-universal catalysts for hydrogen evolution at high current density

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A universal synthesis strategy to make metal nitride electrocatalysts for hydrogen evolution reaction

Luo Yu et al.

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Promoting nitrogen electroreduction to ammonia with bismuth nanocrystals and potassium cations in water

Yu-Chen Hao et al.

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From Two-Phase to Three-Phase: The New Electrochemical Interface by Oxide Electrocatalysts

Zhichuan J. Xu

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From Two-Phase to Three-Phase: The New Electrochemical Interface by Oxide Electrocatalysts

Zhichuan J. Xu

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Cobalt Covalent Doping in MoS2 to Induce Bifunctionality of Overall Water Splitting

Qizhong Xiong et al.

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Water splitting by electrolysis at high current densities under 1.6 volts

Haiqing Zhou et al.

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Direct observation of noble metal nanoparticles transforming to thermally stable single atoms

Shengjie Wei et al.

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CO2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface

Cao-Thang Dinh et al.

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High-performance bifunctional porous non-noble metal phosphide catalyst for overall water splitting

Fang Yu et al.

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Anion insertion enhanced electrodeposition of robust metal hydroxide/oxide electrodes for oxygen evolution

Zhenhua Yan et al.

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Co3O4/Fe0.33Co0.66P Interface Nanowire for Enhancing Water Oxidation Catalysis at High Current Density

Xiaoyan Zhang et al.

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Phosphorus-doped graphene supported palladium (Pd/PG) electrocatalyst for the hydrogen evolution reaction in PEM water electrolysis

S. Shiva Kumar et al.

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Nanostructured NiFe (oxy)hydroxide with easily oxidized Ni towards efficient oxygen evolution reactions

Dazhong Zhong et al.

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Highly Active, Nonprecious Electrocatalyst Comprising Borophene Subunits for the Hydrogen Evolution Reaction

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Activating lattice oxygen redox reactions in metal oxides to catalyse oxygen evolution

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Platinum single-atom and cluster catalysis of the hydrogen evolution reaction

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Under-Water Superaerophobic Pine-Shaped Pt Nanoarray Electrode for Ultrahigh-Performance Hydrogen Evolution

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Ultrathin Spinel-Structured Nanosheets Rich in Oxygen Deficiencies for Enhanced Electrocatalytic Water Oxidation

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Polymer Electrolyte Membrane Electrolyzers Utilizing Non-precious Mo-based Hydrogen Evolution Catalysts

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