4.8 Article

Elastic Plasmonic-Enhanced Fabry-Perot Cavities with Ultrasensitive Stretching Tunability

期刊

ADVANCED MATERIALS
卷 34, 期 7, 页码 -

出版社

WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.202106731

关键词

catalytic activity; Fabry-Perot cavities; plasmon-enhancement; self-embedded arrays; wrinkled surfaces

资金

  1. Ramon y Cajal Fellowship [RyC2013-14479, MCIN/AEI/10.13039/501100011033]
  2. Generalitat de Catalunya [2017-SGR-292]
  3. CERCA programme/Generalitat de Catalunya
  4. Swedish Foundation for Strategic Research (SFF) grant [FFL15-0026, RMX18-0039]
  5. Swedish Government Strategic Research Area in Materials Science on Functional Materials at Linkoping University (Faculty Grant SFO-Mat-LiU) [2009-00971]
  6. [MAT201677391-R]
  7. [PID2019-106229RB-I00]
  8. [PCIN2016-093]
  9. [DPI201568197-R]
  10. [DPI2015-72948-EXP]
  11. [SEV-20170706]
  12. Swedish Foundation for Strategic Research (SSF) [RMX18-0039, FFL15-0026] Funding Source: Swedish Foundation for Strategic Research (SSF)

向作者/读者索取更多资源

The first stretchable plasmonic-enhanced and wrinkled Fabry-Perot (FP) cavities are demonstrated, which are composed of self-embedded arrays of Au nanostructures at controlled depths into elastomer films. These novel structures have unprecedented optomechanical effects and can be used for strain sensing.
The emerging stretchable photonics field faces challenges, like the robust integration of optical elements into elastic matrices or the generation of large optomechanical effects. Here, the first stretchable plasmonic-enhanced and wrinkled Fabry-Perot (FP) cavities are demonstrated, which are composed of self-embedded arrays of Au nanostructures at controlled depths into elastomer films. The novel self-embedding process is triggered by the Au nanostructures' catalytic activity, which locally increases the polymer curing rate, thereby inducing a mechanical stress that simultaneously pulls the Au nanostructures into the polymer and forms a wrinkled skin layer. This geometry yields unprecedented optomechanical effects produced by the coupling of the broad plasmonic modes of the Au nanostructures and the FP modes, which are modulated by the wrinkled optical cavity. As a result, film stretching induces drastic changes in both the spectral position and intensity of the plasmonic-enhanced FP resonances due to the simultaneous cavity thickness reduction and cavity wrinkle flattening, thus increasing the cavity finesse. These optomechanical effects are exploited to demonstrate new strain-sensing approaches, achieving a strain detection limit of 0.006%, i.e., 16-fold lower than current optical strain-detection schemes.

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