4.8 Article

Room-temperature Near-infrared Excitonic Lasing from Mechanically Exfoliated InSe Microflake

期刊

ACS NANO
卷 16, 期 1, 页码 1477-1485

出版社

AMER CHEMICAL SOC
DOI: 10.1021/acsnano.1c09844

关键词

indium selenide; microlasers; near-infrared lasing; exciton-exciton scattering; two-dimensional semiconductors

资金

  1. Natural Science Foundation of China [51991340, 51991344, 52072006]
  2. Strategic Priority Research Program of Chinese Academy of Sciences [XDA25040201]
  3. National Natural Science Foundation of China [51727901]
  4. Key Laboratory for Laser Plasmas (Ministry of Education)
  5. Beijing Natural Science Foundation [JQ18014]
  6. CAS Interdisciplinary Innovation Team

向作者/读者索取更多资源

This study demonstrates room-temperature near-infrared lasing from mechanically exfoliated.-phase indium selenide (InSe) microflakes free from external optical microcavities at a center wavelength of similar to 1030 nm. The lasing action occurs at the sub-Mott density level and is generated by exciton-exciton scattering with a high net modal optical gain of similar to 1029 cm(-1). Microdisks fabricated by a simple laser printing sustain the lasing with a reduced threshold, indicating InSe as a promising material for near-infrared microlasers in various applications.
The development of chip-level near-infrared laser sources using two-dimensional semiconductors is imperative to maintain the architecture of van der Waals integrated optical interconnections. However, the established two-dimensional semiconductor lasers may have either the disadvantages of poor controllability of monolayered gain media, large optical losses on silicon, or complicated fabrication of external optical microcavities. This study demonstrates room-temperature near-infrared lasing from mechanically exfoliated.-phase indium selenide (InSe) microflakes free from external optical microcavities at a center wavelength of similar to 1030 nm. The lasing action occurs at the sub-Mott density level and is generated by exciton-exciton scattering with a high net modal optical gain of similar to 1029 cm(-1). Moreover, the lasing is sustained for microdisks fabricated by a simple laser printing with a reduced threshold. These results suggest that InSe is a promising material for near-infrared microlasers and can be employed in a wide range of applications, including imaging, sensing, and optical interconnects.

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