期刊
ACS APPLIED MATERIALS & INTERFACES
卷 13, 期 51, 页码 60715-60735出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsami.1c13525
关键词
metal organic frameworks; UiO-66; defect engineering; catalysis; catalytic site
资金
- National Natural Science Foundation of China [22101039]
- Chinese Scholarship Council (CSC)
- Ghent University BOF Co-funding grant
- FWO [PEGASUS]2 Marie Sklodowska-Curie Grant [665501]
- Research Board of Ghent University [GOA010-17, BOF GOA2017000303]
- Zhang Dayu School of Chemistry
UiO-66 is considered as an epitome of metal-organic frameworks (MOFs) due to its stability and capability to withstand high numbers of defects without structural collapse. Numerous studies have focused on constructing catalytic sites in UiO-66 through defect engineering to enhance performance.
UiO-66 is regarded as an epitome of metal-organic frameworks (MOFs) because of its stability. Defect engineering has been used as a toolbox to alter the performance of MOFs. UiO-66 is among the most widely explored MOFs because of its capability to bear a high number of defects without undergoing structural collapse. Several representative works in the field of MOF-based defect engineering are available based on UiO-66. In this review, more emphasis is given toward the construction of catalytic sites by engineering defects in UiO-66 as a representative including all the detailed synthesis procedures for inducing defects, and the characterization techniques used to analyze these defects in UiO-66 are discussed. Furthermore, a comprehensive review for the defects themselves and the support using defects in catalysis is provided to accentuate the importance of defect engineering.
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