Promoting Rechargeable Batteries Operated at Low Temperature

Article Chemistry, Multidisciplinary

Regulating Interfacial Chemistry in Lithium-Ion Batteries by a Weakly Solvating Electrolyte**

Yu-Xing Yao et al.

Summary: The research reveals a weakly solvating electrolyte that improves the performance of Li-ion batteries by forming unique anion-derived interfaces, demonstrating fast-charging and long-term cycling characteristics.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Research Progress of Lithium Plating on Graphite Anode in Lithium-Ion Batteries

Daozhong Hu et al.

Summary: Lithium plating on graphite anode is accelerated by fast charge and low temperature, leading to degradation of the battery's state of health (SOH) and potential safety risks. Various methods such as anode surface modification, electrolyte optimization, and charge strategy development are discussed to suppress lithium plating. Remaining challenges include mechanism research, detection methods, and further development of suppression techniques.

CHINESE JOURNAL OF CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Inhibiting Solvent Co-Intercalation in a Graphite Anode by a Localized High-Concentration Electrolyte in Fast-Charging Batteries

Li-Li Jiang et al.

Summary: By utilizing a localized high-concentration electrolyte, a uniform and robust solid electrolyte interphase can be achieved on the graphite surface, leading to fast-charging performance and excellent cycling stability of lithium-ion batteries.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Review Chemistry, Physical

Insights into the Nanostructure, Solvation, and Dynamics of Liquid Electrolytes through Small-Angle X-Ray Scattering

Kun Qian et al.

Summary: Understanding the nanostructures of liquid electrolytes is crucial for enhancing electrochemical energy storage capacities, but the solvation structures and molecular dynamics in electrolytes are difficult to probe. Small-angle X-ray scattering (SAXS) offers unique insights into molecular clusters and ion pairs in electrolytes, with excellent time-resolution for studying molecular dynamics. This review focuses on the microscopic understanding of liquid electrolytes by SAXS and highlights the unique capabilities of X-ray scattering for nanostructure characterization.

ADVANCED ENERGY MATERIALS (2021)

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Article Energy & Fuels

Tailoring electrolyte solvation for Li metal batteries cycled at ultra-low temperature

John Holoubek et al.

Summary: This study highlights the importance of the solvation structure of the electrolyte in charge-transfer behavior at ultra-low temperatures for lithium metal batteries. By designing an electrolyte to enable low-temperature operations, stable performance and high efficiency can be achieved for Li-metal batteries.

NATURE ENERGY (2021)

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Article Nanoscience & Nanotechnology

Novel Low-Temperature Electrolyte Using Isoxazole as the Main Solvent for Lithium-Ion Batteries

Sha Tan et al.

Summary: A novel electrolyte system with improved low-temperature performance for lithium-ion batteries has been developed by utilizing isoxazole as the main solvent, resulting in significantly higher ionic conductivity and reversible capacity at -20 degrees C.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Physical

Revisiting the designing criteria of advanced solid electrolyte interphase on lithium metal anode under practical condition

Shouyi Yuan et al.

Summary: The research found that the organic composition in the SEI layer determines the Coulombic Efficiency of LMBs, and designing the SEI layer by adjusting the electrolyte composition may improve battery performance. An advanced multilayer SEI layer was designed in carbonate electrolyte, demonstrating potential for high energy density and long cycle life.

NANO ENERGY (2021)

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Article Chemistry, Physical

Enabling the Low-Temperature Cycling of NMC∥Graphite Pouch Cells with an Ester-Based Electrolyte

Yoon-Gyo Cho et al.

Summary: Utilizing an ester electrolyte based on methyl propionate, LiNixMnyCozO2 parallel graphite full cells demonstrate successful cycling at high rates at extremely low temperatures. This work provides a new avenue for achieving high-performance LIBs capable of ultralow-temperature charging and discharging operations.

ACS ENERGY LETTERS (2021)

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Article Chemistry, Multidisciplinary

All-Climate Iron-Based Sodium-Ion Full Cell for Energy Storage

Yongjie Cao et al.

Summary: A novel carbon-coated iron-based borate anode material shows excellent performance in sodium-ion batteries with high reversible specific capacity and good cycling stability, capable of operating over a wide temperature range.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

An Atomic Insight into the Chemical Origin and Variation of the Dielectric Constant in Liquid Electrolytes

Nan Yao et al.

Summary: The dielectric constant is a crucial physicochemical property of liquids, which changes with temperature and electrolyte compositions. Solvent dielectric constants decrease as temperatures rise, and for solvent mixtures, they either follow a linear superposition rule or satisfy a polynomial function.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Copper Zinc Tin Sulfide Anode Materials for Lithium-Ion Batteries at Low Temperature

Zeru Syum et al.

Summary: Developing novel materials, such as copper zinc tin sulfide (CZTS) thin film with nanowalls structure, as an anode material in thin-film LIBs for low-temperature applications, shows higher reversible capacity compared to traditional graphite electrodes. The improved interfacial stability and Li+ diffusion of CZTS contribute to its enhanced cycling performance in low temperatures.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2021)

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Article Multidisciplinary Sciences

An organic/inorganic electrode-based hydronium-ion battery

Zhaowei Guo et al.

NATURE COMMUNICATIONS (2020)

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Review Chemistry, Physical

Fundamentals and Challenges of Lithium Ion Batteries at Temperatures between-40 and 60 °C

Junbo Hou et al.

ADVANCED ENERGY MATERIALS (2020)

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Article Chemistry, Physical

Solid-State Proton Battery Operated at Ultralow Temperature

Lei Yan et al.

ACS ENERGY LETTERS (2020)

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Article Chemistry, Physical

Advanced Electrolytes for Fast-Charging High-Voltage Lithium-Ion Batteries in Wide-Temperature Range

Xianhui Zhang et al.

ADVANCED ENERGY MATERIALS (2020)

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Article Chemistry, Physical

An All-Fluorinated Ester Electrolyte for Stable High-Voltage Li Metal Batteries Capable of Ultra-Low-Temperature Operation

John Holoubek et al.

ACS ENERGY LETTERS (2020)

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Article Chemistry, Multidisciplinary

Zinc-Organic Battery with a Wide Operation-Temperature Window from-70 to 150 °C

Nan Wang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Low-Temperature Charge/Discharge of Rechargeable Battery Realized by Intercalation Pseudocapacitive Behavior

Xiaoli Dong et al.

ADVANCED SCIENCE (2020)

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Article Chemistry, Physical

Efficient Low-Temperature Cycling of Lithium Metal Anodes by Tailoring the Solid-Electrolyte Interphase

Akila C. Thenuwara et al.

ACS ENERGY LETTERS (2020)

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Article Energy & Fuels

Low-temperature and high-rate-charging lithium metal batteries enabled by an electrochemically active monolayer-regulated interface

Yue Gao et al.

NATURE ENERGY (2020)

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Article Chemistry, Physical

A High-Rate Aqueous Proton Battery Delivering Power Below-78 °C via an Unfrozen Phosphoric Acid

Heng Jiang et al.

ADVANCED ENERGY MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Fluorinated carboxylate ester-based electrolyte for lithium ion batteries operated at low temperature

Yang Yang et al.

CHEMICAL COMMUNICATIONS (2020)

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Article Chemistry, Physical

Energizing hybrid supercapacitors by using Mn2+-based active electrolyte

Lei Yan et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Article Chemistry, Multidisciplinary

Salt-rich solid electrolyte interphase for safer high-energy-density Li metal batteries with limited Li excess

Shouyi Yuan et al.

CHEMICAL COMMUNICATIONS (2020)

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Article Electrochemistry

A High-Rate and Long-Life Rechargeable Battery Operated at -75°C

Xiaoli Dong et al.

BATTERIES & SUPERCAPS (2020)

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Article Chemistry, Physical

A metal-free battery working at -80 °C

Jian Qin et al.

ENERGY STORAGE MATERIALS (2020)

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Article Chemistry, Multidisciplinary

High-Energy Rechargeable Metallic Lithium Battery at-70°C Enabled by a Cosolvent Electrolyte

Xiaoli Dong et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Chemistry, Physical

Graphite-based lithium ion battery with ultrafast charging and discharging and excellent low temperature performance

Jiang Xu et al.

JOURNAL OF POWER SOURCES (2019)

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Article Energy & Fuels

Monolithic solid-electrolyte interphases formed in fluorinated orthoformate-based electrolytes minimize Li depletion and pulverization

Xia Cao et al.

NATURE ENERGY (2019)

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Article Chemistry, Multidisciplinary

Aqueous Batteries Operated at-50 °C

Qingshun Nian et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Chemistry, Multidisciplinary

Exploiting Mechanistic Solvation Kinetics for Dual-Graphite Batteries with High Power Output at Extremely Low Temperature

John Holoubek et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Energy & Fuels

All-temperature batteries enabled by fluorinated electrolytes with non-polar solvents

Xiulin Fan et al.

NATURE ENERGY (2019)

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Article Multidisciplinary Sciences

Synergistic Effects of Salt Concentration and Working Temperature towards Dendrite-Free Lithium Deposition

Panlong Li et al.

RESEARCH (2019)

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Article Nanoscience & Nanotechnology

Dual Lithiophilic Structure for Uniform Li Deposition

Shouyi Yuan et al.

ACS APPLIED MATERIALS & INTERFACES (2019)

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Article Chemistry, Physical

Extending the low temperature operational limit of Li-ion battery to -80 °C

Jiang Xu et al.

ENERGY STORAGE MATERIALS (2019)

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Article Chemistry, Multidisciplinary

A versatile single-ion electrolyte with a Grotthuss-like Li conduction mechanism for dendrite-free Li metal batteries

Shouyi Yuan et al.

ENERGY & ENVIRONMENTAL SCIENCE (2019)

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Article Chemistry, Physical

High-Efficiency Lithium-Metal Anode Enabled by Liquefied Gas Electrolytes

Yangyuchen Yang et al.

JOULE (2019)

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Article Electrochemistry

Factors Limiting Li+ Charge Transfer Kinetics in Li-Ion Batteries

T. Richard Jow et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2018)

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Article Chemistry, Physical

Designing Low Impedance Interface Films Simultaneously on Anode and Cathode for High Energy Batteries

Bo Liao et al.

ADVANCED ENERGY MATERIALS (2018)

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Article Chemistry, Physical

Organic Batteries Operated at -70 degrees C

Xiaoli Dong et al.

JOULE (2018)

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Article Multidisciplinary Sciences

Liquefied gas electrolytes for electrochemical energy storage devices

Cyrus S. Rustomji et al.

SCIENCE (2017)

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Article Chemistry, Multidisciplinary

A Simple Prelithiation Strategy To Build a High-Rate and Long-Life Lithium-Ion Battery with Improved Low-Temperature Performance

Yao Liu et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2017)

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Review Chemistry, Multidisciplinary

Computational Exploration of the Li-ElectrodelElectrolyte Interface in the Presence of a Nanometer Thick Solid-Electrolyte Interphase Layer

Yunsong Li et al.

ACCOUNTS OF CHEMICAL RESEARCH (2016)

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Article Multidisciplinary Sciences

Lithium-ion battery structure that self-heats at low temperatures

Chao-Yang Wang et al.

NATURE (2016)

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Article Electrochemistry

The use of ethyl acetate as a sole solvent in highly concentrated electrolyte for Li-ion batteries

R. Petibon et al.

ELECTROCHIMICA ACTA (2015)

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Review Chemistry, Multidisciplinary

Electrolytes and Interphases in Li-Ion Batteries and Beyond

Kang Xu

CHEMICAL REVIEWS (2014)

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Article Electrochemistry

Lithium-Ion Electrolytes Containing Ester Cosolvents for Improved Low Temperature Performance

M. C. Smart et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2010)

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Article Chemistry, Physical

Solvation sheath of Li+ in nonaqueous electrolytes and its implication of graphite/electrolyte interface chemistry

Kang Xu et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2007)

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Article Chemistry, Physical

Molecular dynamics simulations of lithium alkyl carbonates

Oleg Borodin et al.

JOURNAL OF PHYSICAL CHEMISTRY B (2006)

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Review Chemistry, Multidisciplinary

Nonaqueous liquid electrolytes for lithium-based rechargeable batteries

K Xu

CHEMICAL REVIEWS (2004)

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Review Chemistry, Multidisciplinary

Liquid fragility and the glass transition in water and aqueous solutions

CA Angell

CHEMICAL REVIEWS (2002)

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Promoting Rechargeable Batteries Operated at Low Temperature

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