期刊
GREEN CHEMISTRY
卷 18, 期 10, 页码 2941-2945出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6gc00362a
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资金
- National Natural Science Foundation of China [21202138]
- Xiangtan University Academic Leader Program [11QDZ20]
- New Teachers' Fund for Doctor Stations, Ministry of Education [20124301120007]
- Hunan Provincial Natural Science Foundation [13JJ4047]
- Hunan Provincial Excellent Young Scientist Foundation [13B114]
- University Student Innovation Program [2014xtuxj18]
A convenient metal-free cascade oxidative decarbonylative alkylarylation of acrylamides with aliphatic aldehydes to provide quaternary oxindoles is developed. With DTBP as an oxidant and radical-initiator, this reaction efficiently converts cheap and abundant aliphatic aldehydes into valuable alkyl radicals for the cascade construction of C(sp(3))-C(sp(3)) and C(sp(3))-C(sp(2)) bonds via dual C(sp(2))-H bond functionalization.
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