期刊
ACS APPLIED ENERGY MATERIALS
卷 4, 期 8, 页码 7487-7491出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsaem.1c01158
关键词
calcium-ion batteries; intercalation; potassium vanadium bronze; calcium vanadium bronze; cathode material
资金
- Samsung Research Funding & Incubation Center of Samsung Electronics [SRFC-MA1601-04]
- Creative Materials Discovery Program through the National Research Foundation of Korea - Ministry of Science, ICT and Future Planning [2015M3D1A1069707]
The research presents K0.5V2O5 as a cathode material for CIBs, showing a high reversible discharge capacity at room temperature. The findings demonstrate the potential for developing high-capacity crystal-water-free cathode materials for CIBs.
The research to discover a suitable cathode material for calcium-ion batteries (CIBs) remains challenging, despite their potential advantages of high energy density and cost-effectiveness. Herein, we report K0.5V2O5 as a cathode material for CIBs. During the initial charging of the electrode, potassium ions were replaced with 0.12 Ca. The calcium-exchanged electrode exhibited a reversible discharge capacity of similar to 100 mAh g(-1) at 0.1 C rate at room temperature with an average voltage of similar to 3.0 V (vs Ca/Ca2+). The reversible capacity is higher than any reported cathode materials without crystal water, demonstrating the feasibility of further development of high-capacity crystal-water-free CIB cathode materials.
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