期刊
JOULE
卷 5, 期 9, 页码 2479-2503出版社
CELL PRESS
DOI: 10.1016/j.joule.2021.06.015
关键词
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资金
- U.S. Department of Energy (DOE) [DE-AC36-08GO28308]
- US Department of Energy, Office of Energy Efficiency and Renewable Energy
- US Department of Energy, Advanced Manufacturing Office (AMO)
- US Department of Energy, Bioenergy Technologies Office (BETO)
- AMO
- BETO
- National Renewable Energy Laboratory (NREL)
- NREL [DE-AC36-08GO28308]
- Research England (E3 scheme)
Esterases play a crucial role in enzymatic PET recycling, enabling efficient depolymerization to TPA and ethylene glycol, reducing energy consumption and greenhouse gas emissions, and generating more socio-economic benefits.
Esterases have emerged as important biocatalysts for enzyme-based polyester recycling of poly(ethylene terephthalate) (PET) to terephthalic acid (TPA) and ethylene glycol (EG). Here, we present process modeling, techno-economic, life-cycle, and socioeconomic impact analyses for an enzymatic PET depolymerization-based recycling process, which we compare with virgin TPAmanufacturing. We predict that enzymatically recycled TPA (rTPA) can be cost-competitive and highlight key areas to achieve this. In addition to favorable long-term socioeconomic benefits, rTPA can reduce total supply chain energy use by 69%-83% and greenhouse gas emissions by 17%-43% per kg of TPA. An economy-wide assessment for the US estimates that the TPA recycling process can reduce environmental impacts by up to 95% while generating up to 45% more socioe-conomic benefits, also relative to virgin TPA production. Sensitivity analyses highlight impactful research opportunities to pursue toward realizing biological PET recycling and upcycling.
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