☆ 4.7 Review

Application of MXenes in Perovskite Solar Cells: A Short Review

NANOMATERIALS (2021)

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Tuning the reactivity of PbI2 film via monolayer Ti3C2Tx MXene for two-step-processed CH3NH3PbI3 solar cells

Yu Zhao et al.

Summary: In this study, 2D monolayer Ti3C2Tx MXene nanosheets were introduced into the PbI2 layer to enhance reactivity and convert it to perovskite efficiently. The Ti3C2Tx additive also improved the energy-level alignment of the perovskite and passivated defects effectively, leading to a champion power conversion efficiency of 19.27%.

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Hysteresis Analysis of Hole-Transport-Material-Free Monolithic Perovskite Solar Cells with Carbon Counter Electrode by Current Density-Voltage and Impedance Spectra Measurements

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Summary: Organic-inorganic perovskite solar cells have attracted attention due to their increased power conversion efficiency, but current density-voltage hysteresis remains a key challenge. Establishing a measurement protocol for reliable results is necessary. Hysteresis was found to be dependent on scan direction and time delay, with impedance spectroscopy revealing further insights into the effects of scan speed, delay, and frequency. Studies on hysteresis could help improve device performance and stability in the long term.

NANOMATERIALS (2021)

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Article Energy & Fuels

2D Materials as Electron Transport Layer for Low-Temperature Solution-Processed Perovskite Solar Cells

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Summary: Low-temperature solution-processed perovskite solar cells are cost-effective and efficient, but face challenges in scalability. 2D materials are gaining attention in the PSC community for their tunable bandgap and high carrier mobility, but further research is needed for their application in PSCs.

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Single-Layered MXene Nanosheets Doping TiO2 for Efficient and Stable Double Perovskite Solar Cells

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Summary: The study introduced a simple strategy of doping single-layered MXene nanosheets into titania as a multifunctional electron transport layer for Cs2AgBiBr6 double perovskite solar cells, significantly improving device performance and stability.

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Efficient perovskite solar cells via improved carrier management

Jason J. Yoo et al.

Summary: Metal halide perovskite solar cells have shown great potential to disrupt the silicon solar cell market with their improved performance, yet still face limitations in light-harvesting due to charge carrier recombination. Efforts to enhance charge carrier management offer a path to increase device performance and approach the theoretical efficiency limit of PSCs.

NATURE (2021)

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Efficient Two-Dimensional Perovskite Solar Cells Realized by Incorporation of Ti3C2Tx MXene as Nano-Dopants

Xin Jin et al.

Summary: 2D Ti3C2T MXene nanosheets with high electrical conductivity and mobility were used as a nanosized additive to enhance the performance of 2D perovskite films, resulting in improved crystallinity, orientation, and charge transfer speed, leading to increased efficiency of solar cells.

NANO-MICRO LETTERS (2021)

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MXenes for Solar Cells

Lujie Yin et al.

Summary: The application of two-dimensional MXene materials in photovoltaics has attracted attention for their unique properties, and this review focuses on the development and applications of Ti3C2Tx MXene in solar cells. Existing problems are discussed and suggestions for further exploration are provided to advance the research in this area.

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A Brief Review of High Efficiency III-V Solar Cells for Space Application

J. Li et al.

Summary: The demands for space solar cells are continuously increasing due to the requirements for higher efficiency and better radiation resistance. III-V multijunction solar cells have become the main focus for space application nowadays, as they possess high efficiency and superb radiation resistance. New materials and structures with high efficiency are continuously developed, featuring low-cost, lightweight, flexible, and high power-to-mass ratio characteristics.

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Compositional and Interfacial Engineering Yield High-Performance and Stable p-i-n Perovskite Solar Cells and Mini-Modules

Janardan Dagar et al.

Summary: Through optimization of perovskite precursor composition and interfaces, a p-i-n-type perovskite solar cell with 22.3% power conversion efficiency was achieved, demonstrating a new performance record. The high device performance is attributed to improved perovskite absorber quality, increased open-circuit voltage with reduced recombination losses, and high-quality hole-selective contacts. Long-term stability of devices was maintained using additives and optimized deposition methods, with scaled-up device architecture achieving high efficiency mini-modules.

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Multifunctional Magnetic Ti3C2Tx MXene/Graphene Aerogel with Superior Electromagnetic Wave Absorption Performance

Luyang Liang et al.

Summary: The study successfully developed a three-dimensional dielectric/magnetic aerogel with superior absorption performance, broad absorption bandwidth, and excellent electromagnetic wave absorbing capabilities, demonstrating potential for stable and durable electromagnetic applications.

ACS NANO (2021)

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MXene in the lens of biomedical engineering: synthesis, applications and future outlook

Adibah Zamhuri et al.

Summary: MXene is a multifaceted 2D material with unique physicochemical properties and biocompatibility, suitable for applications in biomedicine and biotechnology such as drug delivery and bio-imaging.

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Recovery of Pure Silicon and Other Materials from Disposed Solar Cells

Lineesh Punathil et al.

Summary: This research focuses on efficiently recovering pure silicon and other materials such as aluminium, silver, and lead from disposed solar cells using chemical treatments. By eliminating the usage of highly toxic and corrosive hydrofluoric acid, pure silicon (99.9984%) has been successfully recovered by sequentially treating with three different chemicals. Aluminum, silver, and lead are also recovered as aluminum hydroxide, silver chloride, and lead oxide, respectively.

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A brief review of hole transporting materials commonly used in perovskite solar cells

Song Li et al.

Summary: Perovskite solar cells (PSCs) have gained significant attention in the field of photovoltaics due to their exceptional performance, with the power conversion efficiency reaching up to 25.2%. This review focuses on discussing various hole transporting materials (HTMs) in PSCs, emphasizing their role in improving photovoltaic performance. Different organic and inorganic HTMs are categorized and their advantages and disadvantages are demonstrated, with the aim of providing insights for the design and application of novel HTMs to further enhance PSCs performance.

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Transition metal carbides (MXenes) for efficient NiO-based inverted perovskite solar cells

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Summary: This work demonstrates the beneficial role of MXene doping in NiO-based inverted perovskite solar cells, improving charge extraction and collection efficiency to achieve superior performance. The ability to finely tune MXene work function during chemical synthesis and modify optoelectronic properties of PSC layers as dopant opens up countless possibilities for engineering inverted PSC structures.

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Review of Interface Passivation of Perovskite Layer

Yinghui Wu et al.

Summary: Perovskite solar cells are a promising substitute for silicon-based solar cells, but their power conversion efficiency and stability need to be improved. Practical interface engineering techniques have been introduced to enhance the efficiency and stability of organic-inorganic lead halide PSCs, focusing on addressing defects at the interface and modifying the perovskite layers with different materials for long-term stability.

NANOMATERIALS (2021)

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Lead-free tin perovskite solar cells

Tianhao Wu et al.

Summary: Efficient and stable development of lead-free perovskite solar cells (PSCs) using tin as a promising candidate for high-performance, eco-friendly photovoltaic technology has been reviewed. Approaches toward efficiency improvement and challenges in reaching higher PCE and scalable production for tin PSCs have been discussed in this paper with the goal of accelerating their commercialization.

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Summary: Incorporating 2D MXenes into the electron transporting layer of perovskite solar cells has been shown to deliver high-efficiency photovoltaic devices. By employing metallic single-walled carbon nanotubes to prepare composites, a power conversion efficiency of over 21% is achieved, demonstrating a new avenue for realizing high-performance PSCs.

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Jinyi Sui et al.

Summary: Transition metal carbides or nitrides (MXene) have shown promising applications in energy conversion and storage (ECS) due to their high conductivity and adjustable surface functional groups. Different morphologies of MXene derivatives, including 0D quantum dots, 1D nanoribbons, 2D nanosheets, and 3D nanoflowers, have demonstrated impressive performance in photocatalysis, electrocatalysis, and rechargeable batteries. Despite their potential, MXene derivatives still face challenges in ECS, which require further research and solutions.

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Facile synthesis of MXene-supported copper oxide nanocomposites for catalyzing the decomposition of ammonium perchlorate

Keding Li et al.

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MXenes: An Emerging Platform for Wearable Electronics and Looking Beyond

Neng Li et al.

Summary: Wearable devices have potential applications in various fields, but the development of flexible wearable electronics is still in its early stages. MXenes, as wonder materials, have shown promise in energy storage and sensing applications across different research areas.

MATTER (2021)

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Article Chemistry, Multidisciplinary

Modulation of perovskite crystallization processes towards highly efficient and stable perovskite solar cells with MXene quantum dot-modified SnO2

Yingguo Yang et al.

Summary: The study explores the modulation of perovskite crystallization kinetics by nanocrystalline SnO2 layers, showing that MQDs-SnO2 layer can rapidly induce perovskite nucleation and improve the crystal quality and phase stability. With superior charge extraction properties, the corresponding PSCs achieved up to 23.3% steady-state power conversion efficiency and outstanding stability against humidity and light soaking.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Article Chemistry, Physical

Performance improvement of MXene-based perovskite solar cells upon property transition from metallic to semiconductive by oxidation of Ti3C2Tx in air

Lin Yang et al.

Summary: By oxidizing Ti3C2Tx, its properties can be adjusted for use as an electron transport layer in low-temperature processed perovskite solar cells (PSCs), resulting in improved energy conversion efficiency. Heavy oxidation of Ti3C2Tx reduces macroscopic defects in the film and transitions it from a metallic material to a semiconductor, leading to enhanced electron mobility and reduced electron-hole recombination for higher power conversion efficiency (PCE).

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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MXene and MBene as efficient catalysts for energy conversion: roles of surface, edge and interface

Si Zhou et al.

Summary: MXenes and MBenes, as part of a two-dimensional transition metal carbides family, have attracted tremendous attention in recent years due to their diverse chemical properties in renewable energy applications. They exhibit superior electrical conductivity, high hydrophility, and outstanding stability, showing promising prospects for applications. The roles of the surface, edge, and interface of these two-dimensional nanostructures in energy conversion have been discussed.

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