期刊
ADVANCED OPTICAL MATERIALS
卷 9, 期 17, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adom.202100544
关键词
broadband emission; low-dimensional structures; perovskites; photoluminescence; single crystals
资金
- National Key R&D Program of China [2019YFB1503200]
- National Natural Science Foundation of China [U2001214]
- Fundamental Research Funds for the Central Universities [SWU 119067]
- NSF of Guangdong Province [2019B151520050]
- GDUPS(2016)
Low-dimensional metal-halide single crystals, particularly the zero-dimensional materials, have shown promising light emission properties with broad luminescence spectra and high color rendition. Despite the strong quantum confinement and electron-phonon coupling, the exploration of 0D structures remains limited.
The high-profile candidacy of low-dimensional metal-halide single crystals as promising light emitters originates from the intriguing emission properties (e.g., extremely broad luminescence spectra, large Stokes shift, high color rendition), which have enabled the recent great achievements on their application in lighting, artificial illumination, and scintillators. Among the family of low-dimensional metal-halide single crystals, zero-dimensional (0D) materials have been featured in the lowest dimensionality, and as a consequence, strongest quantum confinement, softest lattice, and strongest electron-phonon coupling have been further translated into near-unity photoluminescence (PL) efficiency with broadband emission. However, as far as it is known, 0D structures are significantly underexplored. Herein, an overview is provided on recent advances of 0D metal-halide single crystals, with a focus on comprehensive understanding and insightful perspectives behind the photophysical mechanism. Additionally, the challenges and future opportunities currently faced by 0D bulk metal halides are discussed in order to provide a roadmap for the future development of novel materials with versatile optical properties suited for practical applications.
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