Frequency stabilization of a quantum cascade laser by weak resonant feedback from a Fabry-Perot cavity

Frequency-stabilized mid-infrared lasers are valuable tools for precision molecular spectroscopy. However, their implementation remains limited by complicated stabilization schemes. Here we achieve optical self-locking of a quantum cascade laser to the resonant leak-out field of a highly mode-matched two-mirror cavity. The result is a simple approach to achieving stable frequencies from high-powered mid-infrared lasers. For short time scales (<0.1 ms), we report a linewidth reduction factor of 3 x 10(-6) to a linewidth of 12 Hz. Furthermore, we demonstrate two-photon cavity-enhanced absorption spectroscopy of an N2O overtone transition near a wavelength of 4.53 mu m. (C) 2021 Optical Society of America

Automated summary

Frequency-stabilized mid-infrared lasers are important for precision molecular spectroscopy, but complex stabilization schemes have limited their implementation. This study demonstrates optical self-locking of a quantum cascade laser to a two-mirror cavity, resulting in stable frequencies with significant linewidth reduction. Additionally, two-photon cavity-enhanced absorption spectroscopy of an N2O overtone transition near a wavelength of 4.53 um was successfully carried out.