期刊
OPTICS EXPRESS
卷 29, 期 14, 页码 21936-21946出版社
OPTICAL SOC AMER
DOI: 10.1364/OE.427232
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资金
- National Natural Science Foundation of China [11827806, 11874368]
The study investigates the mechanism of low-order harmonic generation induced by a strong laser field, with a focus on the third harmonic generation. It is found that the third harmonic generation is strongly suppressed in counter-rotating bi-chromatic laser fields, and the quantum-mechanical treatment provides a better explanation for experimental observations compared to the semi-classical photocurrent model. The work suggests that overlapping in continuum states via different quantum paths of a single electron plays a role in low-order harmonic generation under elliptical bi-chromatic laser fields.
The low-order harmonic generation induced by a strong laser field produces a bright, ultrashort, supercontinuum radiation ranging from the terahertz to ultraviolet band. By controlling the phase-delay and ellipticity of the bi-chromatic laser fields, the third harmonic generation is experimentally and theoretically investigated for elucidating the mechanism of the low-order harmonics. The third harmonic generation is found to be strongly suppressed in the counter-rotating bi-chromatic laser field due to the selection rule for harmonic emissions. The continuum-continuum transition in the strong field approximation is extended to explain the third harmonic generation as a function of the phase delay and ellipticity of the bi-chromatic laser fields. Compared with the semi-classical photocurrent model, the continuum-continuum transition on the basis of quantum-mechanical treatment achieves better agreement with the experimental observations. Our work indicates that the overlapping in continuum states via different quantum paths of a single electron plays a role in low-order harmonics generation under elliptical bi-chromatic laser fields. (C) 2021 Optical Society of America under the terms of the OSA Open Access Publishing Agreement
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