4.8 Article

Perovskite semiconductors for room-temperature exciton-polaritonics

期刊

NATURE MATERIALS
卷 20, 期 10, 页码 1315-1324

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NATURE PORTFOLIO
DOI: 10.1038/s41563-021-01035-x

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资金

  1. National Natural Science Foundation of China [12020101003, 52072006]
  2. Tsinghua University start-up grant
  3. Singapore Ministry of Education [MOE2018-T3-1-002, MOE2019-T2-1-004, MOE2018-T2-2-068]
  4. Agence Nationale de la Recherche [ANR-18-CE24-0016, ANR-17-CE24-0020]
  5. IDEXLYON from Universite de Lyon, Scientific Breakthrough project TORE within the Programme Investissements d'Avenir [ANR-19-IDEX-0005]
  6. project PRIN Interacting Photons in Polariton Circuits-INPhoPOL (MIUR) Accordo bilaterale CNR/RFBR (Russia) - triennio 2021-2023 [2017P9FJBS_001]
  7. Agence Nationale de la Recherche (ANR) [ANR-17-CE24-0020] Funding Source: Agence Nationale de la Recherche (ANR)

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Lead-halide perovskites show great promise for exciton-polariton studies and polaritonic devices operating at room temperature. Recent rapid experimental advances have been made using lead-halide perovskites, but challenges and mysteries remain in pushing polaritons to room-temperature operation.
An outlook on the potential of lead-halide perovskites as a playground for exciton-polariton studies and for the development of polaritonic devices operating at room temperature is provided. Lead-halide perovskites are generally excellent light emitters and can have larger exciton binding energies than thermal energy at room temperature, exhibiting great promise for room-temperature exciton-polaritonics. Rapid progress has been made recently, although challenges and mysteries remain in lead-halide perovskite semiconductors to push polaritons to room-temperature operation. In this Perspective, we discuss fundamental aspects of perovskite semiconductors for exciton-polaritons and review the recent rapid experimental advances using lead-halide perovskites for room-temperature polaritonics, including the experimental realization of strong light-matter interaction using various types of microcavities as well as reaching the polariton condensation regime in planar microcavities and lattices.

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