4.8 Article

Volcanic relationship between wettability of the interface and water migration rate in solar steam generation systems

期刊

NANO RESEARCH
卷 15, 期 2, 页码 1238-1245

出版社

TSINGHUA UNIV PRESS
DOI: 10.1007/s12274-021-3631-5

关键词

solar water steam generation; surface interface reaction; wettability; volcanic relationship; computational modeling

资金

  1. National Natural Science Foundation of China [21871009, 21527803]
  2. Youth Science Foundation of Hubei University [202011303000002]
  3. China Postdoctoral Science Foundation [2018M641064]

向作者/读者索取更多资源

Understanding the mechanism of water molecules interacting with the interface is crucial for the performance of solar water treatment devices. Research shows that different wettability of interfaces can affect water evaporation performance, leading to a double-edged sword effect on device performance.
Capturing solar energy as heat for water treatment has become a substantial approach to obtain freshwater. To obtain higher performance, the understanding of the mechanism of how water molecules interact with the interface is particularly fundamental, because the migration process of water molecules on the evaporation interface will directly affect the performance of the device. Herein we regulate the number of hydroxyl groups on the surface of reduced graphene oxide quantitatively, to study the effect of different wettability of interfaces on the performance of solar water generators. The water evaporation performance displays a volcanic shape as increasing wettability. Calculated by the computational chemistry method, deviation from proper wetting humidity is not conducive to the migration of water molecules from the surface. The double-edged sword effect of wettability on performances is clarified, and the surface energy density is the key to break through the limit by the finite element method.

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