4.6 Article

Bubble Manipulation Driven by Alternating Current Electrowetting: Oscillation Modes and Surface Detachment

期刊

LANGMUIR
卷 37, 期 23, 页码 6898-6904

出版社

AMER CHEMICAL SOC
DOI: 10.1021/acs.langmuir.1c00096

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资金

  1. Science and Technology Program of Guangzhou [201904020007, 2019050001]
  2. Grant of 2019 Guangdong recruitment program of foreign experts [191900022]
  3. Program for Guangdong Innovative and Entrepreneurial Teams [2019BT02C241]
  4. Program for Chang Jiang Scholars and Innovative Research Teams in Universities [IRT_17R40]
  5. Guangdong Provincial Key Laboratory of Optical Information Materials and Technology [2017B030301007]
  6. Guangzhou Key Laboratory of Electronic Paper Displays Materials and Devices [201705030007]
  7. MOE International Laboratory for Optical Information Technologies
  8. 111 Project
  9. Natural Science Foundation of Guangdong Province [2021A1515010623]

向作者/读者索取更多资源

This study investigates the manipulation of millimeter-sized bubbles in water using the electrowetting on dielectric technique, where standing waves on the bubble surface and three resonance peaks are observed. By incorporating the nonlinear friction force and conducting simulations, it is found that low-frequency resonance peaks are associated with bubble detachment due to inertial effects. The experimental detachment process is well-reproduced in the simulations, confirming the role of fluid inertia in bubble detachment.
In this paper, a millimeter-sized bubble in water pending on a substrate is manipulated by applying an alternating current (AC) electric field, known as electrowetting on dielectric. In this setup, standing waves on the bubble surface are observed. The amplitude of these waves varies with frequency, and three resonance peaks (21, 76, and 134 Hz) can be identified. By incorporating the nonlinear friction force for the contact line to an existing surface mode model, a significant improvement to explain the spectrum of the oscillations is obtained, predicting three peak positions, widths, and heights with good accuracy. We also show that bubble detachment correlates with the low-frequency resonance peak. It is found experimentally that if close enough to this peak, then bubbles at sufficiently high voltages are observed to detach from the substrate. This suggests that inertial effects can effectively promote bubble detachment. To confirm this hypothesis, the bubble dynamics is simulated with COMSOL using the full Navier-Stokes equation with a two-phase field and electrostatic stresses. It was found that the bubble experimental detachment process is quite well-reproduced in the simulation, confirming the role of fluid inertia for the detachment process. Given the nice correspondence between the experimental state diagrams and the theoretical modeling, this work contributes to identify a window for precise and reliable bubble manipulation by means of AC electrowetting.

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