期刊
LANGMUIR
卷 37, 期 23, 页码 6947-6952出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.langmuir.1c00437
关键词
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资金
- National Natural Science Foundation of China [61927814, 51875544, 51675503, 91963127]
- National Key R&D Program of China [2017YFB1104303]
- Major Scientific and Technological Projects in Anhui Province [201903a05020005]
- Fundamental Research Funds for the Central Universities [YD209000205, WK6030000108, WK5290000001, WK2090050048]
- Youth Innovation Promotion Association CAS [2017495]
- Experimental Center of Engineering and Material Sciences at USTC
Aeration is a mass transfer process that disperses gas into a liquid, typically using a microporous device. The surface wettability of the gas/solid interface significantly affects bubble size, which is often overlooked. A superhydrophilic/superhydrophobic Janus aluminum foil fabricated by laser microstructuring improves gas dissolution rate and has broad applications in wastewater treatment, energy production, and aquaculture.
Aeration is a mass transfer process, in which gas is dispersed into a liquid by utilizing air inflation or agitation. Typically, a microporous device is often used for aeration. Increasing the gas flow rate and decreasing the pore size reduce the bubble size, but the surface wettability of the gas/solid interface also has a significant impact on the bubble size, which is rarely studied. In this study, a superhydrophilic/superhydrophobic Janus aluminum foil (JAF) is fabricated by laser microstructuring and low surface energy modification. The gas-repelling superhydrophilic surface not only facilitates ultrafine bubble generation but also allows the bubbles to detach from the aerator surface quickly, while the superhydrophobic surface prevents water from infiltrating into the aeration chamber and reduces the mass transfer resistance. The micropores with different diameters are obtained by adjusting the laser processing parameters. The pore prepared by the laser is uniform, consequently leading to the uniform bubble size. When the pore diameter is set to 30 mu m, the diameter of bubbles released from the superhydrophilic surface of the JAF is only 0.326 mm, and the gas dissolution rate is about six times that of the double-sided superhydrophobic aluminum foil. This simple, low-cost, and controllable method of the laser processing JAF has broad applications in wastewater treatment, energy production, and aquaculture.
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