期刊
JOURNAL OF THE EUROPEAN CERAMIC SOCIETY
卷 41, 期 16, 页码 101-112出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.jeurceramsoc.2021.09.027
关键词
Pack cementation; Ceramic matrix composite; Bond coat; SiC; Oxidation
资金
- MTU Aero Engines AG
- German Federal Ministry for Economic Affairs and Energy (BMWi) [LuFo 5/3 Ker_Twk]
The potential and limitations of a halide-activated pack cementation process for the development of bond coats on SiC/SiC Ceramic Matrix Composites were investigated. A two-step pack cementation process using chromium and aluminum was proposed to achieve an alumina-forming coating, which protected the fiber-matrix interface from oxidation.
The potentials and limitations of a halide-activated pack cementation process on SiC/SiC Ceramic Matrix Composites for the development of bond coats as part of environmental barrier coating (EBCs) systems were investigated. Different pack compositions using chromium, aluminum and alloys of these elements were tested and the kinetics of coating formation were examined in addition to their microstructure. The results and their analogy to diffusion couples were discussed and it was shown that coating elements which form silicides and carbides are promising candidates for coatings deposited on SiC/SiC via pack cementation. Based on such considerations a two-step pack cementation was proposed, which used chromium, one of the suitable elements, in a first step, to finally achieve an alumina-forming coating. The oxidation resistance of the developed coating was tested via thermogravimetric analysis and compared to the uncoated material. The coating protected the fiber-matrix interface of the SiC/SiC Ceramic Matrix Composites from oxidation.
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