期刊
JOURNAL OF MOLECULAR LIQUIDS
卷 334, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.molliq.2021.116063
关键词
CuO/g-C3N4-NS; Layer nanostructure; Primary amides; CuO nanorods; Green synthesis
An intelligent strategy for fabricating CuO nanorods-decorated graphitic carbon nitride nanosheets was developed for the synthesis of primary amides in water. The morphology of CuO and its synergistic effect with g-C3N4 played a significant role in product yield, while NH2OH·HCl was used as a substitute for ammonia source. The nanostructured catalyst showed excellent performance in converting aldehyde derivatives to corresponding amides, providing new insights in organic transformation.
Herein, we describe an intelligent strategy to fabricate nanosheets of graphitic carbon nitride (g-C3N4) decorated with nanorods copper oxide (CuO NRs). Then, the catalytic activity of CuONRs/g-C3N4-NS was developed for the synthesis of primary amides in water. The morphology of CuO and its synergetics effect with nanosheets g-C3N4 a major role in the yield of products. Furthermore, hydroxylamine hydrochloride (NH2OH center dot HCl) due to availability and affordability was used as a suitable substitute for ammonia source. The findings demonstrate that this layer nanostructure is a superb catalyst for converting various derivatives of aldehyde to their corresponding amides. The current protocol can be useful criterion in the synthesis and stabilization of metal oxides and provides new insight in organic transformation. (C) 2021 Elsevier B.V. All rights reserved.
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