期刊
JOURNAL OF HAZARDOUS MATERIALS
卷 416, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.jhazmat.2021.126217
关键词
CeO2; Cr(VI) reduction; Z-scheme
资金
- Natural Science Research of Jiangsu Higher Education Institutions of China [20KJB610018]
- Jiangsu Province Industry-University-Research Cooperation Project [BY2020629]
- Jiangsu Agriculture Science and Technology Innovation Fund [CX(20)3169]
- Yancheng Teachers University [72061871011C]
- Jiangsu province Undergraduate Innovation and Entrepreneurship training program [202010324051Y]
- 2019 Jiangsu Science and Technology Association Young Talents Lifting Project
The SnIn4S8/CeO2 (SISC) composites fabricated by a stirring and calcination method show promising photocatalytic activity under visible light, with good degradation effect on hexavalent chromium (Cr (VI)) and high hydrogen production efficiency.
Semiconductor photocatalysis technology is a promising method for hydrogen production and water pollution treatment. Here, the SnIn4S8/CeO2 (SISC) composites were fabricated by a stirring and calcination method, and the mass ratio of SnIn4S8 to CeO2 was optimized. The 50 wt% SISC heterojunction photocatalyst has the highest visible light catalytic activity. The degradation rate of hexavalent chromium (Cr (VI)) is 98.8% in 75 min of light irradiation, which is 2.48 times that of pure CeO2. Besides, the 50 wt% SISC composite photocatalyst also has the highest photocatalytic hydrogen production efficiency (0.6193 mmol g-1 h-1), which exhibits a higher photocatalytic activity than pure CeO2 and SnIn4S8. The enhanced photocatalytic performance can be attributed to the Z-scheme heterojunction structure between CeO2 and SnIn4S8, which can effectively separate and transfer photogenerated charges, thereby reducing the recombination of photo-generated carriers. We hope this work can provide ideas for constructing Z-scheme heterojunction structures and improving photocatalytic activity under visible light.
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