4.7 Article

Comparative environmental benefits of power generation from underground and surface coal gasification with carbon capture and storage

期刊

JOURNAL OF CLEANER PRODUCTION
卷 310, 期 -, 页码 -

出版社

ELSEVIER SCI LTD
DOI: 10.1016/j.jclepro.2021.127383

关键词

Underground coal gasification; Underground gasification combined cycle; Life cycle assessment; Environmental benefit; Carbon capture and storage

资金

  1. National Key R&D Program of China [2016YFA0602603]
  2. National Natural Science Foundation of China [71521002, 71622012, 71673026]

向作者/读者索取更多资源

This study assessed the environmental impacts of UGCC with and without CCS through life cycle assessment, revealing that UGCC power plants have lower mid-point impact values but higher global warming potential compared to IGCC power plants. Additionally, UGCC power plants show superior end-point environmental benefits, but the implementation of CCS may result in an increase in damage to ecosystem quality and resources.
Underground gasification combined cycle (UGCC), when combined with carbon capture and storage (CCS), is widely judged to be a promising approach for clean coal utilization especially in the context of carbon neutral energy pathways. Nevertheless, the overall operation processes may consume a multiple of energy and inevitably trigger environmental concerns. Hence, a careful evaluation of the potential environmental impacts associated with UGCC is needed. In this study, we assessed environmental impacts of UGCC with and without CCS by the life cycle assessment method, and compared the results with those of surface integrated gasification combined cycle (IGCC) to gain better insight into tradeoffs of two coal gasification technologies and lighten the environmental burden by design optimizations. The results demonstrated that most mid-point impact values of UGCC power plants, which reflect pollution emissions and corresponding damage degree, were lower. Inversely, the global warming potential was 16.9% higher than those of IGCC power plants. Furthermore, UGCC power plants have superior end-point environmental benefits, which represent the damage of ecosystem quality, human health and resources. As demonstrated by the fact that the value of above three impact types were 23%, 15% and 4%, lower than those of IGCC power plants, respectively. In addition, the implement of CCS in two types of power plants decreased human health damage due to reduced greenhouse gas emissions, but notable environmental trade-offs are the increase in ecosystem quality damage and resource damage. The aggregated results show that UGCC with or without CCS has a more outstanding environmental performance with exception of global warming potential than IGCC with or without CCS. Enhancing UCG process control, improving syngas heating value and decreasing the energy in gasification agent preparation are effective methods to further reduce the GHG emissions. Approached in an improved way, UGCC-CCS stands to provide a low-carbon and self-contained solution for power production and energy provision.

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