Optical two-dimensional coherent spectroscopy of many-body dipole-dipole interactions and correlations in atomic vapors

Many-body interactions and correlations in atomic ensembles are fundamental in understanding many-body effects such as collective and emergent phenomena and also play an important role in various atom-based applications. Optical two-dimensional coherent spectroscopy (2DCS) provides a powerful tool to measure many-body interactions and correlations. Here, we present the study of many-body dipole-dipole interactions and correlations in potassium and rubidium atomic vapors by using double-quantum and multi-quantum 2DCS. The results show that double-quantum 2DCS provides sensitive and background-free detection of weak dipole-dipole interaction between atoms with a mean separation up to about 16 mu m, and multi-quantum 2DCS can excite and detect multi-atom states (Dicke states) with up to eight correlated atoms. The technique of optical 2DCS can provide a new approach to study many-body physics in atomic ensembles and can be potentially implemented to measure many-body effects in cold atoms and other atomic/molecular systems.

Automated summary

Optical two-dimensional coherent spectroscopy is a powerful tool for studying many-body interactions and correlations in atomic ensembles, providing sensitive and background-free detection of weak dipole-dipole interactions and multi-atom states. This technique has the potential to measure many-body effects in cold atoms and other atomic/molecular systems.