Thermocapillary deformation induced by laser heating of thin liquid layers: Physical and numerical experiments

Characterizing the profile of the laser-induced thermocapillary deformation of a thin liquid layer on a laser absorbing solid is of great fundamental and applied importance. The thermocapillary effect is the basis of several non-contact methods for measuring the physicochemical and thermal properties of liquids and solids, and methods of non-destructive testing in material science and thermal physics. The study of the layer rupturing caused by laser beam heating could contribute to solving the problem of the dry spots formation in thin-film heat exchangers. In this regard, the development of physical and numerical tools to determine the thermocapillary profiles of thin liquid layers is of great interest to researchers. In the present work, we developed a home-made setup to scan a deformed surface of a liquid layer with a laser sheet. Its accuracy was verified by scanning the surface of a solid standard specimen with a given Gaussian profile. By scanning the thermocapillary deformed layers of silicone oil, we found that for the Gaussian distribution of the radiation intensity in the heating laser beam, the thermocapillary deformations are significantly not the Gaussian. A modified Agnesi function, which is characterized by high accuracy and allows defining the surface profile using a minimum of experimental data, is shown to be an optimal function for approximating the thermocapillary deformation. Using Agnesi approximation can significantly reduce the time of the experiment and the processing of results. To validate new experimental data, an axisymmetric numerical model of the thermocapillary convection in a thin liquid layer was developed using commercial software Comsol Multiphysics. It helped calculating the surface profile and the temperature field on the substrate for two boundary conditions of radiative heat exchange in the system corresponding to maximum and minimum radiation heat loss. For the case of the ebonite-silicone oil system, when the laser beam is absorbed by the ebonite surface, it was numerically shown that the difference between the types of boundary conditions becomes noticeable only on very thin layers close to the pseudo-rupture. In general, a comparison of the stationary profiles of the thermocapillary surface deformation and temperature distributions obtained experimentally and numerically for the entire range of the studied layer thicknesses shows satisfactory agreement between the physical and numerical results. (C) 2021 Elsevier Ltd. All rights reserved.

Automated summary

Characterizing laser-induced thermocapillary deformation has significant importance in measuring physicochemical properties, solving dry spots formation, and thermal physics. Using the modified Agnesi function can significantly reduce experiment time and result processing efficiency.