4.6 Article

Gas-Liquid Taylor Flow Characteristics in a Fractal Microchannel Network during Numbering-up and Sizing-up

期刊

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
卷 60, 期 21, 页码 7935-7949

出版社

AMER CHEMICAL SOC
DOI: 10.1021/acs.iecr.1c00448

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资金

  1. Youth Innovation Promotion Association of Chinese Academy of Sciences
  2. Frontier Scientific Research Project - Shell [PT19253]
  3. STS Program of Chinese Academy of Sciences [KFJJ-STS-SCYD-302]

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In this study, the characteristics of gas-liquid Taylor flow in a fractal microchannel network were investigated using numerical modeling and experiments. Significant size effects were observed in different sized channels, with changes in gas-liquid flow rate ratios affecting slug and bubble lengths. The stability of the flow pattern deteriorated at high gas velocities, with swirling vortices observed in the liquid slug.
In the present study, the characteristics of gas-liquid Taylor flow in a fractal microchannel network were investigated by numerical modeling and experiments. With perpendicular gas intake, the fractal design methodology resulted in uniform flow distribution. Unstable Taylor flow and saddle-shaped velocity profile were observed in a high-level branch with 0.3 mm width. The liquid slug exhibited different flow fields during splitting in the bifurcations of different levels. The significant size effects were further investigated in four channels representing different sizes (0.3, 0.6, 1.2, and 2.4 mm) via a mu-PIV and high-speed camera. The normalized slug length (L-S/W) increased with the increasing gas-liquid flow rate ratio (j(G)/j(L)), while the bubble length (L-B/W) followed an opposite trend. The stability of the gas-liquid Taylor flow pattern became worse when the gas velocity increased beyond a certain value (Reynolds number Re > 220) under the microscale effect. Two typical counter rotating vortices were observed in the liquid slug, and the swirling strength increased exponentially with the j(G)/j(L). It was found that both the velocity profile in the 0.3 mm channel deviated from the laminar flow. Particularly, a flow field similar to turbulence was observed in the 0.3 mm channel when the j(G)/j(L) reached 4. This work quantified the significant size effect in micro- and millichannels, providing theoretical basis for the effective scale-up of the microreactor.

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