期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 27, 期 55, 页码 13669-13698出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.202101587
关键词
covalent-organic frameworks; composites; electrochemistry; energy conversion; lithium-ion battery
资金
- SERB-DST, New Delhi, India [CRG/2020/001769]
- CSIR [01(2935)/18/EMR-II]
- BRNS, Mumbai, India [58/14/17/2020-BRNS/37215]
- IIT Indore
- CSIR-JRF fellowships
- MHRD, India
- UGC-JRF fellowship
- DST-Inspire fellowships
Covalent-organic frameworks (COFs) as a new member of the crystalline porous materials family have emerged as important materials for energy storage/conversion/generation devices, thanks to their high surface areas, ordered micro/mesopores, designable structures, and ability to precisely control electro-active groups in their pores which broaden their application window. They have been found suitable for a range of challenging electrochemical applications due to their low weight density, long range crystallinity, reticular nature, and tunable synthesis approach towards two and three dimensional (2D and 3D) networks.
Covalent-organic frameworks (COFs), being a new member of the crystalline porous materials family, have emerged as important materials for energy storage/conversion/generation devices. They possess high surface areas, ordered micro/mesopores, designable structures and an ability to precisely control electro-active groups in their pores, which broaden their application window. Thanks to their low weight density, long range crystallinity, reticular nature and tunable synthesis approach towards two and three dimensional (2D and 3D) networks, they have been found suitable for a range of challenging electrochemical applications. Our review focuses on the progress made on the design, synthesis and structure of COFs and their composites for various energy applications, such as metal-ion batteries, supercapacitors, water-splitting and solar cells. Additionally, attempts have been made to correlate the structural and mechanistic characteristics of COFs with their applications.
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