期刊
CATALYSIS COMMUNICATIONS
卷 156, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.catcom.2021.106318
关键词
Activated carbon; P-doping; Dehydroaromatization; Phosphorus source; n-Hexane
Phosphorus-doped activated carbon (P@AC) can serve as an efficient metal-free catalyst for the dehydroaromatization of n-hexane to benzene under mild conditions. The active sites for dehydroaromatization catalysis are believed to be functional groups containing -P(O)(OH) on the carbon surface, as indicated by characterization analysis.
Phosphorus-doped activated carbon (P@AC), prepared by wet impregnation method, can serve as efficient metalfree catalyst for the dehydroaromatization of n-hexane to benzene under mild conditions. The effect of phosphorus amount and phosphorus sources including phenylphosphonic acid (PPOA), phosphorus acid (H3PO4), triphenylphosphine (TPP), and tributylphosphine (TBP) on catalytic performance of P@AC were investigated. Combining with characterization analysis, functional groups containing -P(O)(OH) on the carbon surface are believed to be the active sites for dehydroaromatization catalysis.
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