期刊
ACS APPLIED MATERIALS & INTERFACES
卷 13, 期 23, 页码 27419-27429出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsami.1c04741
关键词
conjugated polymer; sebaceous fingerprint; blood fingerprint; adaptive; fluorescence; fingerprint development
资金
- China Academy of Engineering [2020-YZ-01]
- Major Basic Research Project of the Natural Science Foundation of the Jiangsu Higher Education Institutions of China [18KJA430014]
- Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD)
The new adaptive fingerprint developing strategy utilizes a synthesized polymer with an appropriate solvent to efficiently develop different types of fingerprints, providing more possibilities for forensic investigations.
Both latent sebaceous and blood fingerprints may provide valuable information for forensic investigation. To detect both types of fingerprints with no need to predistinguish them, a new adaptive developing strategy was proposed. A cationic conjugated polymer with poly[p-(phenylene ethylene)-alt-(thienylene ethynylene)] backbone (PPETE-NMe3+) was synthesized, which was dissolved in N,N-dimethylformamide (DMF) to form the developing solution. Fingerprints were developed by a simple dropping and incubating process without any pre-/post-treatments. Fluorescent photographs of the developed fingerprints on various substrates demonstrated that this developing strategy was effective for both types of fingerprints on nonporous substrates. Gray value analysis further confirmed the enhancement of the legibility of the fingerprint images. The preliminary mechanism exploration suggested that certain weak interactions, such as hydrophobic interaction and electrostatic interaction, may synergistically contribute to the interaction between the polymer and fingerprint components. The molecular design of the polymer combined with an appropriate solvent endowed the developing system the adaptiveness toward different types of fingerprints. This adaptive developing strategy made the fingerprint-developing process more efficient and may be further extended to more practical application scenes.
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