☆ 4.8 Article

New Insights into the Mechanism of LiDFBOP for Improving the Low-Temperature Performance via the Rational Design of an Interphase on a Graphite Anode

ACS APPLIED MATERIALS & INTERFACES (2021)

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Review Chemistry, Physical

A Growing Appreciation for the Role of LiF in the Solid Electrolyte Interphase

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Summary: Rechargeable lithium batteries have transformed energy storage technology, but their further commercialization is hindered by short lifetime and safety issues, mainly due to the unstable solid-electrolyte interphase (SEI) and uncontrolled lithium dendrite growth. Research on SEI worldwide has focused on its debated structure and composition, particularly the role of the main component LiF. This review covers the development history of the SEI model, fundamental understanding of SEI, categorization of anode materials generating LiF in SEI, characterization techniques of SEI layers, transport mechanism of Li+ ions within SEI, physical properties of LiF, and analysis of LiF sources, offering insights for future research directions to promote large-scale applications of lithium metal batteries.

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