4.6 Article

Frustration-driven magnetic fluctuations as the origin of the low-temperature skyrmion phase in Co7Zn7Mn6

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NPJ QUANTUM MATERIALS
卷 6, 期 1, 页码 -

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NATURE PORTFOLIO
DOI: 10.1038/s41535-021-00342-5

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资金

  1. SNSF Sinergia [CRSII5_171003]
  2. JSPS [20K15164]
  3. JST CREST [JPMJCR1874, JPMJCR20T1]
  4. EU [730872]
  5. Swiss National Science Foundation (SNF) [CRSII5_171003] Funding Source: Swiss National Science Foundation (SNF)
  6. Grants-in-Aid for Scientific Research [20K15164] Funding Source: KAKEN

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This study reveals a direct correlation between the stability of the second skyrmion phase in the chiral magnet Co7Zn7Mn6 and an underlying magnetic fluctuation rate driven by geometric magnetic frustration. It shows weak influences of other leading skyrmion stability mechanisms in this system, and suggests a fundamental mechanism for stabilizing topological skyrmions drawing upon magnetic frustration.
In chiral cubic helimagnets, phases of magnetic skyrmions-topologically protected spin whirls-are stabilized by thermal fluctuations over a narrow region directly below the magnetic ordering temperature T-c. Due to often being touted for use in applications, there is a high demand to identify new ways to stabilize equilibrium skyrmion phases far below T-c where they may display an enhanced robustness against external perturbation due to a larger magnetic order parameter. Here, from quantum beam experiments on the chiral magnet Co7Zn7Mn6, we unveil a direct correlation between the stability of its second skyrmion phase-stable far from T-c, and a concomitant enhancement of an underlying magnetic fluctuation rate that is driven by geometric magnetic frustration. The influences of other leading skyrmion stability mechanisms, such as those derived from thermal fluctuations and low T cubic anisotropies, are shown to be weak in this system. We therefore advance the existence of a fundamental mechanism for stabilizing topological skyrmions in Co7Zn7Mn6 chiral magnet that draws upon magnetic frustration as the key ingredient.

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