4.6 Article

Topologically driven linear magnetoresistance in helimagnetic FeP

期刊

NPJ QUANTUM MATERIALS
卷 6, 期 1, 页码 -

出版社

NATURE RESEARCH
DOI: 10.1038/s41535-021-00337-2

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资金

  1. National Science Foundation Division of Materials Research [DMR-1905891]
  2. Gordon and Betty Moore Foundation's EPiQS Initiative [GBMF9071]
  3. National Science Foundation [DMR-1157490, 1644779]
  4. state of Florida
  5. Anne G. Wylie Dissertation Fellowship
  6. Maryland NanoCenter and its FabLab
  7. Foundation for Polish Science through the International Research Agendas program
  8. European Union
  9. Direct For Mathematical & Physical Scien
  10. Division Of Materials Research [1644779] Funding Source: National Science Foundation

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FeP is a member of the family of binary pnictide materials with the MnP-type structure, exhibiting an anomalously linear magnetoresistance behavior in high magnetic fields. By comparing quantum oscillation frequencies to electronic structure calculations, a semi-Dirac point related to band structure was identified in this system, which disperses linearly perpendicular to the field direction.
The helimagnet FeP is part of a family of binary pnictide materials with the MnP-type structure, which share a nonsymmorphic crystal symmetry that preserves generic band structure characteristics through changes in elemental composition. It shows many similarities, including in its magnetic order, to isostructural CrAs and MnP, two compounds that are driven to superconductivity under applied pressure. Here we present a series of high magnetic field experiments on high-quality single crystals of FeP, showing that the resistance not only increases without saturation by up to several hundred times its zero-field value by 35 T, but that it also exhibits an anomalously linear field dependence over the entire range when the field is aligned precisely along the crystallographic c-axis. A close comparison of quantum oscillation frequencies to electronic structure calculations links this orientation to a semi-Dirac point in the band structure, which disperses linearly in a single direction in the plane perpendicular to field, a symmetry-protected feature of this entire material family. We show that the two striking features of magnetoresistance-large amplitude and linear field dependence-arise separately in this system, with the latter likely due to a combination of ordered magnetism and topological band structure.

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