期刊
EXPOSURE AND HEALTH
卷 14, 期 2, 页码 219-238出版社
SPRINGER
DOI: 10.1007/s12403-021-00391-y
关键词
Arsenic pollution; Groundwater quality; Kriging interpolation; Correlation analysis; Yellow River; Health risk
资金
- National Natural Science Foundation of China [42072286, 41761144059]
- Fundamental Research Funds for the Central Universities of CHD [300102299301]
- Fok Ying Tong Education Foundation [161098]
- China Postdoctoral Science Foundation [2016M590911, 2017T100719]
- Shaanxi Postdoctoral Science Foundation [2016BSHTDZZ03]
- Ten Thousand Talents Program [W03070125]
The main water chemical type in the study area is SO4·Cl-Ca·Mg, followed by HCO3-Ca·Mg type, with rock weathering being the main process influencing the water chemical characteristics. The content of arsenic in groundwater is lower in the dry season and higher in the wet season, with relatively small differences in areas with intense surface water percolation.
High arsenic (As) groundwater is a serious environmental problem in Yinchuan Plain, northwest China. Though some measures have been taken to alleviate it, the detection rate of high As in groundwater is still high. In order to understand the occurrence and enrichment of As in groundwater and the hydrochemical evolution, correlation analysis and interpolation approach were used to interpret the spatiotemporal variation of major ions and contaminants in phreatic groundwater at 30 sampling sites during the dry season (March) and wet season (July). Some suggestions on the treatment of groundwater As pollution in the study area were put forward. The results reveal that the predominant hydrochemical type of groundwater in the study area is SO4 center dot Cl-Ca center dot Mg, followed by HCO3-Ca center dot Mg type, and rock weathering is the main process regulating the hydrochemical characteristics. The content of groundwater As is low in the dry season but high in the wet season. However, the difference of As concentration between the dry and wet seasons is relatively small in the areas where surface water percolation is intense. The concentrations of HCO3-, NH4+, PO43-, and Mn have a significantly positive correlation with the As enrichment in the dry season, while HCO3-, Fe, and Mn have a strongly negative correlation with As in the wet season. The content of As in surface water influences greatly to the As enrichment in groundwater. In the dry season, high arsenic is enriched in areas close to surface water, while in the wet season, the infiltration of irrigation water makes arsenic expand to the western agricultural irrigation area. The mean lung cancer risk caused by As is higher than the maximum acceptable level in the study area. As such, necessary actions such as adopting nanocomposites as As removal material are to be carried out.
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