期刊
NANOMATERIALS
卷 11, 期 4, 页码 -出版社
MDPI
DOI: 10.3390/nano11040893
关键词
copper mesh; ammonia; activated graphene; supercapacitor
类别
资金
- Basic Research Program through the National Research Foundation of Korea (NRF) - Ministry of Science and ICT [2019R1A2C2089785]
- Korea Electric Power Corporation [R19XO01-16]
- National Research Foundation of Korea [2019R1A2C2089785] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
In this study, a porous Cu mesh was utilized as a current collector to investigate its morphological effect on supercapacitor performance. The porous surface was achieved through thermal annealing with ammonia gas. Hierarchically porous activated graphene (AG) was deposited on the P-Cu mesh, resulting in high specific capacitance and energy density due to efficient electric double-layer formation and charge transport. This work presents an alternative approach to enhance supercapacitors by combining a porous metallic current collector with porous AG.
A porous Cu (P-Cu) mesh was used as a current collector and its morphological effect on the supercapacitor performance was investigated. A porous surface was obtained by thermally annealing the Cu mesh using ammonia gas. Hierarchically porous activated graphene (AG) with a high specific surface area (SSA) was deposited on the P-Cu mesh using electrophoretic deposition, aided by graphene oxide (GO). GO was thermally converted to electrically conductive reduced graphene oxide (rGO). The AG/rGO that was deposited on the P-Cu mesh achieved a high specific capacitance of up to 140.0 F/g and a high energy density of up to 3.11 Wh/kg at a current density of 2 A/g in 6 m KOH aqueous electrolyte. The high SSA of AG and the porous surface morphology of the Cu mesh allowed efficient electric double-layer formation and charge transport. This work offers an alternative to improve supercapacitors by combining a porous metallic current collector with porous AG.
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