期刊
ACS PHOTONICS
卷 8, 期 4, 页码 1007-1012出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsphotonics.0c01917
关键词
photonics; color centers; hexagonal boron nitride; 2D materials; stimulated emission depletion
类别
资金
- Engineering and Physical Sciences Research Council [EP/S001557/1, EP/026656/1]
- EPSRC [EP/S001557/1] Funding Source: UKRI
The study demonstrates the use of STED spectroscopy to map the characteristics of color centers in hexagonal boron nitride. A red-shift in the phonon spectra of ground state and excited state was observed. The experimental results suggest a correlation with carbon-based defects.
We demonstrate the use of Stimulated Emission Depletion (STED) spectroscopy to map the electron-optical-phonon sideband of the ground state of the radiative transition of color centers in hexagonal boron nitride emitting at 2.0-2.2 eV, with in-plane linear polarization. The measurements are compared to photoluminescence of excitation (PLE) spectra that maps the electron-optical-phonon sideband of the excited state. The main qualitative difference is a red-shift in the longitudinal optical phonon peak associated with E-1u symmetry at the zone center. We compare our results to theoretical work on different defect species in hBN and find they are consistent with a carbon-based defect.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据