4.8 Article

Sub-thermionic, ultra-high-gain organic transistors and circuits

期刊

NATURE COMMUNICATIONS
卷 12, 期 1, 页码 -

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NATURE PORTFOLIO
DOI: 10.1038/s41467-021-22192-2

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资金

  1. National Natural Science Foundation of China [61927808, 61521001, 61734003, 61851401, 91964202, 61861166001, 51861145202, 61821091, 61888102, 61825403, 11922215]
  2. Natural Science Foundation of Jiangsu Province [BK20202005]
  3. Strategic Priority Research Program of Chinese Academy of Sciences [XDB 30000000]
  4. General Research Fund (GRF) [HKU 17264016, HKU 17204517]
  5. Key Laboratory of Advanced Photonic and Electronic Materials, Collaborative Innovation Center of Solid-State Lighting and Energy-Saving Electronics
  6. Fundamental Research Funds for the Central Universities, China

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Utilizing solution-processed monolayer organic crystal, ferroelectric HfZrOx gating, and van der Waals fabrication, researchers have developed flexible OTFTs with high transconductance and low power consumption. These OTFTs demonstrate outstanding intrinsic gain and amplifier voltage gain, outperforming existing technologies. Additionally, researchers have successfully integrated wearable ECG and pulse sensors with high fidelity amplification, capable of detecting weak ECG waves and diagnosing arrhythmia, showing great promise for battery/wireless-powered applications like electronic skins and RFID tags.
The development of organic thin-film transistors (OTFTs) with low power consumption and high gain will advance many flexible electronics. Here, by combining solution-processed monolayer organic crystal, ferroelectric HfZrOx gating and van der Waals fabrication, we realize flexible OTFTs that simultaneously deliver high transconductance and sub-60 mV/dec switching, under one-volt operating voltage. The overall optimization of transconductance, subthreshold swing and output resistance leads to transistor intrinsic gain and amplifier voltage gain over 5.3 x 10(4) and 1.1 x 10(4), respectively, which outperform existing technologies using organics, oxides and low-dimensional nanomaterials. We further demonstrate battery-powered, integrated wearable electrocardiogram (ECG) and pulse sensors that can amplify human physiological signal by 900 times with high fidelity. The sensors are capable of detecting weak ECG waves (undetectable even by clinical equipment) and diagnosing arrhythmia and atrial fibrillation. Our sub-thermionic OTFT is promising for battery/wireless powered yet performance demanding applications such as electronic skins and radio-frequency identification tags, among many others. Exploiting negative capacitance effects in organic thin-film transistors (OTFTs) is advantageous for enhancing device performance. Here, the authors report solution-processed sub-thermionic OTFTs and circuits with ferroelectric hafnium oxides that show ultra-low power and ultra-high gain.

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