期刊
SURFACE & COATINGS TECHNOLOGY
卷 411, 期 -, 页码 -出版社
ELSEVIER SCIENCE SA
DOI: 10.1016/j.surfcoat.2021.126969
关键词
Thermal barrier coatings (TBCs); Calcium; Magnesium-alumino-silicate (CMAS); Hot corrosion; Cold gas dynamic spray (CGDS); Thermally grown oxide (TGO); Lanthanum zirconate (La2Zr2O7)
资金
- Scientific Research Projects (BAP) Coordinatorship of Bartin University [2017-Fen-A-004]
- Scientific and Technological Research Council of Turkey
- TUBITAK [113R049]
The study investigated the impact of high-temperature oxidation, hot corrosion, and CMAS attacks on YSZ and La2Zr2O7/YSZ TBC systems, revealing that double-layered TBCs provide better durability than traditional YSZ TBCs. Hot corrosion and CMAS attacks significantly damaged the column morphology of the EB-PVD method, reducing the performance of thermal barrier coatings.
Thermal barrier coatings (TBCs) commonly expose to oxidation, hot corrosion, and CaO-MgO-Al2O3-SiO2 (CMAS) attacks during the service condition. All of these attacks cause the spallation or delamination of TBCs from the bond coat. In this study, the effect of these attacks on YSZ and La2Zr2O7/YSZ TBC systems was investigated. YSZ and double layer La2Zr2O7/YSZ topcoats were deposited using electron beam physical technique (EB-PVD) on CoNiCrAlY bond coat produced by cold gas dynamic spray (CGDS) technique. CMAS tests at 1225 degrees C for 4, 8, 12, 16, 20, 24, 28, and 32 h and 5 h cyclic hot corrosion tests at 1000 degrees C were carried out on TBCs. Before and after the tests, TBCs were characterized using scanning electron microscopy (SEM), energy dispersive spectrometer (EDS), x-ray diffraction (XRD) and image analysis software program. At the end of the tests, the formed phases, microstructural changes, and general failure mechanisms were investigated in detail for each test. The general result shows that double-layered TBCs provide significant contributions and durability against high-temperature corrosive attacks of conventional YSZ TBC. In addition, in this study, hot corrosion damage mechanism and CMAS attack significantly damaged the column morphology of the EB-PVD method, reducing the thermal insulation properties and strain tolerance of TBCs. As a result of the tests, spallation and phase changes occurred in the damaged TBC systems.
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