期刊
NANO LETTERS
卷 21, 期 7, 页码 2946-2952出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.1c00055
关键词
Flexoelectric effect; photovoltaic effect; heterostructure; thin film; strain gradient
类别
资金
- National Natural Science Foundation of China (NSFC) [51872148, 51772238]
- Natural Science Foundation of Shandong [ZR2020JQ03]
- CSS project [YK2015-0602006]
- Fundamental research Funds for the Central Universities
- World-Class Universities (Disciplines) and the Characteristic Development Guidance Funds for the Central Universities
- Special Funds of the Taishan Scholar Program of Shandong Province [tsqn201812045]
- Youth Innovation Team Project of Shandong Provincial Education Department [2019KJJ012]
- National University of Singapore
- Singapore Ministry of Education under its Tier 2 Grant [MOE2017-T2-1-129]
- General Research Fund (GRF) of Hong Kong [15300018]
This study presents a flexoelectric photodetector based on a thin-film heterostructure, demonstrating a giant strain gradient in LaFeO3 thin films grown on LaAlO3 substrates, leading to significant flexoelectric polarization and photovoltaic effect with nanosecond response time. This novel self-powered photodetector offers an alternative to traditional interface-type structures and opens up avenues for designing practical flexoelectric devices for nanoelectronics applications.
The flexoelectric effect, which manifests itself as a strain-gradient-induced electrical polarization, has triggered great interest due to its ubiquitous existence in crystalline materials without the limitation of lattice symmetry. Here, we propose a flexoelectric photodetector based on a thin-film heterostructure. This prototypical device is demonstrated by epitaxial LaFeO3 thin films grown on LaAlO3 substrates. A giant strain gradient of the order of 10(6)/m is achieved in LaFeO3 thin films, giving rise to an obvious flexoelectric polarization and generating a significant photovoltaic effect in the LaFeO3-based heterostructures with nanosecond response under light illumination. This work not only demonstrates a novel self-powered photodetector different from the traditional interface-type structures, such as the p-n and Schottky junctions but also opens an avenue to design practical flexoelectric devices for nanoelectronics applications.
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