4.4 Review

A Short Review on Self-Healing Thermoplastic Polyurethanes

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出版社

WILEY-V C H VERLAG GMBH
DOI: 10.1002/macp.202100002

关键词

polyurethane; self‐ healing polymers; thermoplastics

资金

  1. National Key Research and Development Program [2018YFA0703102]
  2. National Natural Science Foundation [51733006]

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Thermoplastic polyurethane (TPU) exhibits high elasticity, tensile strength, and resistance to various conditions, making it suitable for applications in automotive, electronics, medical, coatings, and sports equipment industries. Introduction of self-healing capabilities has significantly improved the service life and recyclability of TPU. Recent research focuses on self-healing supramolecular TPUs, highlighting the importance of balancing mechanical performance and repairability through covalent and non-covalent interactions, while addressing critical issues and challenges associated with this technology.
Thermoplastic polyurethane (TPU) is a melt-processing polymer with a high elasticity, high tensile strength, low-temperature resistance, wear-resistance, and corrosion resistance ability. TPU can be used in the automotive industry, electronics, medical supplies, coatings, and sports equipment. Introduction of self-healing performance has made a considerable contribution to the service life and recyclability of TPU. The present article analyzes recent progress in self-healing supramolecular TPUs. In particular, the importance of self-healing mechanisms governed by covalent bonds and non-covalent interactions in polymer design that allows for balancing mechanical performance and repairability is summarized. The critical issues and challenges associated with self-healing supramolecular TPUs are also discussed.

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