期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 27, 期 30, 页码 8008-8012出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.202100960
关键词
amination; carbazole; electrochemistry; heterocycles; nitrenium ion
资金
- DFG [AN 1064/4-1]
- Boehringer Ingelheim Foundation (Plus 3)
A transition-metal-free direct electrolytic C-H amination involving an electrochemically generated nitrenium ion intermediate has been developed. The electrosynthesis takes place in the absence of any organoiodine catalysts and is enabled by an in situ generated electrolyte. A novel, efficient intramolecular and intermolecular C-H amination has been demonstrated using a simple reaction setup.
A transition-metal-free direct electrolytic C-H amination involving an electrochemically generated nitrenium ion intermediate has been developed. The electrosynthesis takes place in the absence of any organoiodine catalysts and is enabled by an in situ generated electrolyte. A novel, efficient intramolecular and intermolecular C-H amination has been demonstrated using a simple reaction setup.
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