期刊
CARBON
卷 174, 期 -, 页码 248-259出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.carbon.2020.12.005
关键词
CF@PANI@Fe3O4 nanocomposites; Microwave absorber; Lightweight; Low filler content; Attenuation mechanism
资金
- National Natural Science Foundation of China [51672144, 51572137, 51702181, 52072196, 52002199, 52002200]
- Shandong Provincial Key Research and Development Program (SPKRDP) [2019GGX102055]
- Natural Science Foundation of Shandong Province [ZR2019BEM042]
- Innovation and Technology Program of Shandong Province [2020KJA004]
- Taishan Scholars Program of Shandong Province [ts201511034]
A lightweight hybrid nanocomposite with remarkable microwave absorption properties was successfully synthesized in this study, showing great potential for practical applications in the frequency range of 2-18 GHz.
Recently, lightweight has gradually become the most concerned property for a practical microwave absorber in the frequency range of 2-18 GHz. In this work, using commercial carbon fiber (CF) as matrix, the hybrid nanocomposites constructed by CF core, polyaniline (PANI) coating and dispersed Fe3O4 nanoparticles (NPs) were successfully synthesized by the electrodeposition and subsequent hydrothermal process. The systematic characterization results revealed that both PANI and Fe3O4 exerted positive roles in enhancing the microwave absorption properties of bare CF. Under the combined action of various components, the desired products (CF@PANI@Fe3O4 hybrid nanocomposites) exhibited remarkable microwave absorption performances, and the minimal reflection loss (RL) was -46.86 dB at a filler content of 10 wt% and a matching thickness of 2.7 mm. Moreover, a synergistic mechanism was proposed according to multiple reflection/scattering, dipole polarization, interface polarization, eddy current and magnetic resonance, so as to demonstrate the multi-attenuation approaches of the incident electromagnetic wave. (C) 2020 Elsevier Ltd. All rights reserved.
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