期刊
ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
卷 23, 期 18, 页码 18145-18153出版社
SPRINGER HEIDELBERG
DOI: 10.1007/s11356-016-6884-x
关键词
TiO2; Doping; Floatable photocatalyst; Visible light; Diesel oil
资金
- National Natural Science Foundation of China [21277097, 21377095]
- National Natural Science Foundation of China [21277097, 21377095]
TiO2-pearlstone (PS) floatable photocatalysts were synthesized using a facile sol-gel method and confirmed by XRD, N-2 adsorption-desorption, SEM, EDX, TEM, FT-IR, XPS, and UV-vis DRS measurements. It has been found that the photocatalysts composed of anatase TiO2 deposited on the surface of PS and formed mesoporous structure. By N or B/N doping, the band gap of the photocatalyst has been narrowed. The obtained floatable photocatalysts can be applied to solar light-driven remediation of oil-contaminated water. Diesel oil was chosen as the model pollutant to evaluate the photocatalytic activity. The results showed B/N-TiO2-PS exhibited the highest photocatalytic activity for diesel oil under visible light irradiation, which is 48 % removal rate for 9 h. The reaction rate constant k of B/N-TiO2-PS is 0.08423 h(-1), which is four times larger than that of pure TiO2-PS. Moreover, the characteristic of floatable makes the photocatalysts easier to separate and reuse, which showed great potential for practical applications in the field of environmental cleanup and solar energy conversion.
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