期刊
ACS APPLIED MATERIALS & INTERFACES
卷 13, 期 19, 页码 22819-22827出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsami.1c03135
关键词
folding; bilayer MoS2; twist angle; interlayer coupling; moire pattern
资金
- National Natural Science Foundation of China [21903007, 22072006]
- Young Thousand Talents Program [110532103]
- Beijing Normal University [312232102]
- Fundamental Research Funds for the Central Universities [310421109]
- Beijing Municipal Science & Technology Commission [Z191100000819002]
- Basic Science Research Program at the National Research Foundation of Korea [NRF-2017R1A5A1014862, NRF2019R1C1C1003643]
- Basic Science Research Program at the National Research Foundation of Korea - Ministry of Science and ICT [NRF-2021R1C1C2006785]
Constructing a bilayer system with defined twist angles can effectively engineer the physical properties of 2D materials, leading to a new research area of twistronics. This study presents a strategy for the large-scale fabrication of twisted bilayer MoS2, with various twist angles tuning Raman mode frequencies and optical transition energies. The folded bilayers exhibit extremely high photoluminescence with doubled intensity compared to unfolded monolayers, showing potential applications in optoelectronic devices.
Constructing a bilayer system with defined twist angles is an effective way to engineer the physical properties of two-dimensional (2D) materials, opening up a new research area of twistronics. How to achieve high-quality bilayer 2D materials in a controlled and mass production way is of primary importance to this emerging area. In this work, we present a strategy for the large-scale fabrication of twisted bilayer molybdenum disulfide (MoS2) through photolithography patterning and folding of single-crystal monolayer MoS2. Atomic resolution transmission electron spectroscopy directly confirms that the as-achieved folded bilayer MoS2 is of high quality with targeted twist angles. Various twist angles result in tuning Raman mode frequencies and direct optical transition energies. Due to the weak interlayer coupling between the twisted layers, folded bilayers exhibit an extremely high photoluminescence with doubled intensity as compared to the unfolded monolayer, indicating a possible application in optoelectronic devices. Our work provides a new strategy to tailor the properties of MoS2, which will be beneficial to twistable electronics.
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